Observation of Rabi dynamics with a short-wavelength free-electron laser.
Journal
Nature
ISSN: 1476-4687
Titre abrégé: Nature
Pays: England
ID NLM: 0410462
Informations de publication
Date de publication:
08 2022
08 2022
Historique:
received:
13
01
2022
accepted:
08
06
2022
entrez:
17
8
2022
pubmed:
18
8
2022
medline:
20
8
2022
Statut:
ppublish
Résumé
Rabi oscillations are periodic modulations of populations in two-level systems interacting with a time-varying field
Identifiants
pubmed: 35978126
doi: 10.1038/s41586-022-04948-y
pii: 10.1038/s41586-022-04948-y
pmc: PMC9385478
doi:
Types de publication
Journal Article
Research Support, Non-U.S. Gov't
Langues
eng
Sous-ensembles de citation
IM
Pagination
488-493Informations de copyright
© 2022. The Author(s).
Références
Rabi, I. I. Space quantization in a gyrating magnetic field. Phys. Rev. 51, 652–654 (1937).
doi: 10.1103/PhysRev.51.652
Fushman, I. et al. Controlled phase shifts with a single quantum dot. Science 320, 769–772 (2008).
pubmed: 18467584
doi: 10.1126/science.1154643
Vijay, R. et al. Stabilizing Rabi oscillations in a superconducting qubit using quantum feedback. Nature 490, 77–80 (2012).
pubmed: 23038468
doi: 10.1038/nature11505
Feist, A. et al. Quantum coherent optical phase modulation in an ultrafast transmission electron microscope. Nature 521, 200–203 (2015).
pubmed: 25971512
doi: 10.1038/nature14463
Pedrozo-Peñafiel, E. et al. Entanglement on an optical atomic-clock transition. Nature 588, 414–418 (2020).
pubmed: 33328668
doi: 10.1038/s41586-020-3006-1
Autler, S. H. & Townes, C. H. Stark effect in rapidly varying fields. Phys. Rev. 100, 703–722 (1955).
doi: 10.1103/PhysRev.100.703
Ackermann, W. et al. Operation of a free-electron laser from the extreme ultraviolet to the water window. Nat. Photon. 1, 336–342 (2007).
doi: 10.1038/nphoton.2007.76
Emma, P. et al. First lasing and operation of an ångstrom-wavelength free-electron laser. Nat. Photon. 4, 641–647 (2010).
doi: 10.1038/nphoton.2010.176
Ishikawa, T. et al. A compact X-ray free-electron laser emitting in the sub-ångström region. Nat. Photon. 6, 540–544 (2012).
doi: 10.1038/nphoton.2012.141
Allaria, E. et al. Highly coherent and stable pulses from the FERMI seeded free-electron laser in the extreme ultraviolet. Nat. Photon. 6, 699–704 (2012).
doi: 10.1038/nphoton.2012.233
Haroche, S. & Raimond, J.-M. Exploring the Quantum: Atoms, Cavities, and Photons (Oxford Univ. Press Inc, 2006).
Maroju, P. K. et al. Attosecond pulse shaping using a seeded free-electron laser. Nature 578, 386–391 (2020).
pubmed: 32042171
doi: 10.1038/s41586-020-2005-6
Mirian, N. S. et al. Generation and measurement of intense few-femtosecond superradiant extreme-ultraviolet free-electron laser pulses. Nat. Photon. 15, 523–529 (2021).
doi: 10.1038/s41566-021-00815-w
Young, L. et al. Roadmap of ultrafast X-ray atomic and molecular physics. J. Phys. B 51, 032003 (2018).
doi: 10.1088/1361-6455/aa9735
Lindroth, E. et al. Challenges and opportunities in attosecond and XFEL science. Nat. Rev. Phys. 1, 107–111 (2019).
doi: 10.1038/s42254-019-0023-9
Young, L. et al. Femtosecond electronic response of atoms to ultra-intense X-rays. Nature 466, 56–61 (2010).
pubmed: 20596013
doi: 10.1038/nature09177
Rudenko, A. et al. Femtosecond response of polyatomic molecules to ultra-intense hard X-rays. Nature 546, 129–132 (2017).
pubmed: 28569799
doi: 10.1038/nature22373
LaGattuta, K. J. Above-threshold ionization of atomic hydrogen via resonant intermediate states. Phys. Rev. A 47, 1560–1563 (1993).
pubmed: 9909092
doi: 10.1103/PhysRevA.47.1560
Girju, M. G., Hristov, K., Kidun, O. & Bauer, D. Nonperturbative resonant strong field ionization of atomic hydrogen. J. Phys. B 40, 4165–4178 (2007).
doi: 10.1088/0953-4075/40/21/004
Rohringer, N. & Santra, R. Resonant Auger effect at high X-ray intensity. Phys. Rev. A 77, 053404 (2008).
doi: 10.1103/PhysRevA.77.053404
Zhang, S. B. & Rohringer, N. Photoemission spectroscopy with high-intensity short-wavelength lasers. Phys. Rev. A 89, 013407 (2014).
doi: 10.1103/PhysRevA.89.013407
Sako, T. et al. Suppression of ionization probability due to Rabi oscillations in the resonance two-photon ionization of He by EUV free-electron lasers. Phys. Rev. A 84, 053419 (2011).
doi: 10.1103/PhysRevA.84.053419
Kanter, E. P. et al. Unveiling and driving hidden resonances with high-fluence, high-intensity X-ray pulses. Phys. Rev. Lett. 107, 233001 (2011).
pubmed: 22182083
doi: 10.1103/PhysRevLett.107.233001
Fushitani, M. et al. Femtosecond two-photon Rabi oscillations in excited He driven by ultra-short intense laser fields. Nat. Photon. 10, 102–105 (2016).
doi: 10.1038/nphoton.2015.228
Prince, K. C. et al. Coherent control with a short-wavelength free-electron laser. Nat. Photon. 10, 176–179 (2016).
doi: 10.1038/nphoton.2016.13
Rauch, H. et al. Verification of coherent spinor rotation of fermions. Phys. Lett. A 54, 425–427 (1975).
doi: 10.1016/0375-9601(75)90798-7
Nogues, G. et al. Seeing a single photon without destroying it. Nature 400, 239–242 (1999).
doi: 10.1038/22275
Jiang, W.-C., Liang, H., Wang, S., Peng, L.-Y. & Burgdörfer, J. Enhancing Autler–Townes splittings by ultrafast XUV pulses. Phys. Rev. Res. 3, L032052 (2021).
doi: 10.1103/PhysRevResearch.3.L032052
Kramida, A., Ralchenko, Y., Reader, J. & NIST ASD Team NIST Atomic Spectra Database (ver. 5.9) (National Institute of Standards and Technology, 2021).
Chan, W. F., Cooper, G. & Brion, C. E. Absolute optical oscillator strengths for the electronic excitation of atoms at high resolution: experimental methods and measurements for helium. Phys. Rev. A 44, 186–204 (1991).
pubmed: 9905668
doi: 10.1103/PhysRevA.44.186
Žitnik, M. et al. Lifetimes of n
doi: 10.1088/0953-4075/36/20/010
Finetti, P. et al. Pulse duration of seeded free-electron lasers. Phys. Rev. X 7, 021043 (2017).
Greenman, L. et al. Implementation of the time-dependent configuration-interaction singles method for atomic strong-field processes. Phys. Rev. A 82, 023406 (2010).
doi: 10.1103/PhysRevA.82.023406
Eberly, J. H. Area theorem rederived. Opt. Exp. 2, 173–176 (1998).
doi: 10.1364/OE.2.000173
Cohen-Tannoudji, C., Dupont-Roc, J. & Grynberg, G. in Atom–Photon Interactions: Basic Processes and Applications Ch. VI (Wiley, 2004).
Holt, C. R., Raymer, M. G. & Reinhardt, W. P. Time dependences of two-, three-, and four-photon ionization of atomic hydrogen in the ground 1
doi: 10.1103/PhysRevA.27.2971
Rza̧ewsaki, K., Zakrzewski, J., Lewenstein, M. & Haus, J. Strong-field autoionization by smooth laser pulses. Phys. Rev. A 31, 2995–3002 (1985).
Nam, I. et al. High-brightness self-seeded X-ray free-electron laser covering the 3.5 keV to 14.6 keV range. Nat. Photon. 15, 435–441 (2021).
doi: 10.1038/s41566-021-00777-z
Liu, B. et al. The SXFEL upgrade: from test facility to user facility. Appl. Sci. 12, 176 (2022).
doi: 10.3390/app12010176
Svetina, C. et al. The low density matter (LDM) beamline at FERMI: optical layout and first commissioning. J. Synchrotron Radiat. 22, 538–543 (2015).
pubmed: 25931066
pmcid: 4416672
doi: 10.1107/S1600577515005743
Giannessi, L. Overview of PERSEO, a system for simulating FEL dynamics in Mathcad. In Proc. FEL 2006 Conference (eds Abo-Bakr, M. et al.) 91–94 (2006).
Fish, D. A., Brinicombe, A. M., Pike, E. R. & Walker, J. G. Blind deconvolution by means of the Richardson-Lucy algorithm. J. Opt. Soc. Am. A 12, 58–65 (1995).
doi: 10.1364/JOSAA.12.000058
Dey, N. et al. 3D Microscopy Deconvolution using Richardson-Lucy Algorithm with Total Variation Regularization Research Report RR-5272 (INRIA, 2004); https://hal.inria.fr/inria-00070726
Rohringer, N., Gordon, A. & Santra, R. Configuration-interaction-based time-dependent orbital approach for ab initio treatment of electronic dynamics in a strong optical laser field. Phys. Rev. A 74, 043420 (2006).
doi: 10.1103/PhysRevA.74.043420
Bertolino, M., Busto, D., Zapata, F. & Dahlström, J. M. Propensity rules and interference effects in laser-assisted photoionization of helium and neon. J. Phys. B 53, 144002 (2020).
doi: 10.1088/1361-6455/ab84c4
Bertolino, M. & Dahlström, J. M. Multiphoton interaction phase shifts in attosecond science. Phys. Rev. Res. 3, 013270 (2021).
doi: 10.1103/PhysRevResearch.3.013270
Simon, B. The definition of molecular resonance curves by the method of exterior complex scaling. Phys. Lett. 71, 211–214 (1979).
doi: 10.1016/0375-9601(79)90165-8
Tao, L. & Scrinzi, A. Photo-electron momentum spectra from minimal volumes: the time-dependent surface flux method. New J. Phys. 14, 013021 (2012).
doi: 10.1088/1367-2630/14/1/013021
Morales, F., Bredtmann, T. & Patchkovskii, S. iSURF: a family of infinite-time surface flux methods. J. Phys. B 49, 245001 (2016).
doi: 10.1088/0953-4075/49/24/245001