Novel chemically cross-linked self-molding particulate sorbents as solid-phase extraction media.

Binding Chemical reaction Particulate sorbent Solid-phase extraction

Journal

Analytical sciences : the international journal of the Japan Society for Analytical Chemistry
ISSN: 1348-2246
Titre abrégé: Anal Sci
Pays: Switzerland
ID NLM: 8511078

Informations de publication

Date de publication:
May 2023
Historique:
received: 03 07 2022
accepted: 03 08 2022
medline: 25 8 2022
pubmed: 25 8 2022
entrez: 24 8 2022
Statut: ppublish

Résumé

Here, we describe novel, chemically cross-linked, self-molding particulate polymer sorbents that are utilized as a molding-type solid-phase extraction medium (M-SPEM), which exhibits high permeability and rigidness. To fabricate such M-SPEM, first, polyethyleneimine (PEI)-modified reversed-phase (RP)-type particulate sorbents were synthesized, thereafter, they were chemically cross-linked by a polymer having many epoxy groups together with additional PEI. By optimizing the binding conditions of the particulate sorbents, the resultant M-SPEM has almost the same adsorption properties as the corresponding unmolded particulate sorbent for some polar (e.g., uracil and adenine) compounds. The binding technique proposed here is expected to facilitate the fabrication of molding-type sorbents and improve the performance of the SPE procedure.

Identifiants

pubmed: 36001293
doi: 10.1007/s44211-022-00179-3
pii: 10.1007/s44211-022-00179-3
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

749-754

Subventions

Organisme : Japan Society for the Promotion of Science
ID : 20K05571
Organisme : Japan Society for the Promotion of Science
ID : 19H02751

Informations de copyright

© 2022. The Author(s), under exclusive licence to The Japan Society for Analytical Chemistry.

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Auteurs

Yuta Miki (Y)

Department of Applied Chemistry, Aichi Institute of Technology, 1247 Yachigusa, Yakusa-cho, Toyota, 470-0392, Japan.

Hiroya Murakami (H)

Department of Applied Chemistry, Aichi Institute of Technology, 1247 Yachigusa, Yakusa-cho, Toyota, 470-0392, Japan. hmurakami@aitech.ac.jp.

Marin Gotoh (M)

Department of Applied Chemistry, Aichi Institute of Technology, 1247 Yachigusa, Yakusa-cho, Toyota, 470-0392, Japan.

Tomonari Umemura (T)

School of Life Sciences, Tokyo University of Pharmacy and Life Sciences, 1432-1 Horinouchi, Hachioji, 192-0392, Japan.

Yukihiro Esaka (Y)

Gifu Pharmaceutical University, Daigaku-nishi, Gifu, 501-1196, Japan.

Yoshinori Inoue (Y)

Department of Applied Chemistry, Aichi Institute of Technology, 1247 Yachigusa, Yakusa-cho, Toyota, 470-0392, Japan.

Norio Teshima (N)

Department of Applied Chemistry, Aichi Institute of Technology, 1247 Yachigusa, Yakusa-cho, Toyota, 470-0392, Japan.

Classifications MeSH