Torsionally broken symmetry assists infrared excitation of biomimetic charge-coupled nuclear motions in the electronic ground state.


Journal

Chemical science
ISSN: 2041-6520
Titre abrégé: Chem Sci
Pays: England
ID NLM: 101545951

Informations de publication

Date de publication:
17 Aug 2022
Historique:
received: 13 04 2022
accepted: 19 07 2022
entrez: 12 9 2022
pubmed: 13 9 2022
medline: 13 9 2022
Statut: epublish

Résumé

The concerted interplay between reactive nuclear and electronic motions in molecules actuates chemistry. Here, we demonstrate that out-of-plane torsional deformation and vibrational excitation of stretching motions in the electronic ground state modulate the charge-density distribution in a donor-bridge-acceptor molecule in solution. The vibrationally-induced change, visualised by transient absorption spectroscopy with a mid-infrared pump and a visible probe, is mechanistically resolved by

Identifiants

pubmed: 36093002
doi: 10.1039/d2sc02133a
pii: d2sc02133a
pmc: PMC9384489
doi:

Types de publication

Journal Article

Langues

eng

Pagination

9392-9400

Informations de copyright

This journal is © The Royal Society of Chemistry.

Déclaration de conflit d'intérêts

The authors declare no competing interests.

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Auteurs

Gourab Chatterjee (G)

Max Planck Institute for the Structure and Dynamics of Matter Luruper Chaussee 149 22761 Hamburg Germany.

Ajay Jha (A)

Max Planck Institute for the Structure and Dynamics of Matter Luruper Chaussee 149 22761 Hamburg Germany.

Alejandro Blanco-Gonzalez (A)

Department of Chemistry, Bowling Green State University Bowling Green OH 43403 USA olivucci@unisi.it.

Vandana Tiwari (V)

Max Planck Institute for the Structure and Dynamics of Matter Luruper Chaussee 149 22761 Hamburg Germany.
Department of Chemistry, University of Hamburg Martin-Luther-King Platz 6 20146 Hamburg Germany.

Madushanka Manathunga (M)

Department of Chemistry, Bowling Green State University Bowling Green OH 43403 USA olivucci@unisi.it.

Hong-Guang Duan (HG)

Max Planck Institute for the Structure and Dynamics of Matter Luruper Chaussee 149 22761 Hamburg Germany.

Friedjof Tellkamp (F)

Max Planck Institute for the Structure and Dynamics of Matter Luruper Chaussee 149 22761 Hamburg Germany.

Valentyn I Prokhorenko (VI)

Max Planck Institute for the Structure and Dynamics of Matter Luruper Chaussee 149 22761 Hamburg Germany.

Nicolas Ferré (N)

Aix-Marseille Univ, CNRS, ICR 13013 Marseille France.

Jyotishman Dasgupta (J)

Department of Chemical Sciences, Tata Institute of Fundamental Research Mumbai 400005 India.

Massimo Olivucci (M)

Department of Chemistry, Bowling Green State University Bowling Green OH 43403 USA olivucci@unisi.it.
Dipartimento di Biotechnologie, Chimica e Farmacia, Università di Siena I-53100 Siena Italy.

R J Dwayne Miller (RJD)

Departments of Chemistry and Physics, University of Toronto 80 St. George Street Toronto M5S 3H6 Canada dmiller@lphys.chem.utoronto.ca.

Classifications MeSH