Enrofloxacin and Sulfamethoxazole Sorption on Carbonized Leonardite: Kinetics, Isotherms, Influential Effects, and Antibacterial Activity toward

adsorption isotherm adsorption kinetics antibiotic adsorption carbonization elovich enrofloxacin growth inhibition zone intraparticle diffusion leonardite sulfamethoxazole

Journal

Antibiotics (Basel, Switzerland)
ISSN: 2079-6382
Titre abrégé: Antibiotics (Basel)
Pays: Switzerland
ID NLM: 101637404

Informations de publication

Date de publication:
16 Sep 2022
Historique:
received: 20 07 2022
revised: 31 08 2022
accepted: 07 09 2022
entrez: 23 9 2022
pubmed: 24 9 2022
medline: 24 9 2022
Statut: epublish

Résumé

Excessive antibiotic use in veterinary applications has resulted in water contamination and potentially poses a serious threat to aquatic environments and human health. The objective of the current study was to quantify carbonized leonardite (cLND) adsorption capabilities to remove sulfamethoxazole (SMX)- and enrofloxacin (ENR)-contaminated water and to determine the microbial activity of ENR residuals on cLND following adsorption. The cLND samples prepared at 450 °C and 850 °C (cLND450 and cLND550, respectively) were evaluated for structural and physical characteristics and adsorption capabilities based on adsorption kinetics and isotherm studies. The low pyrolysis temperature of cLND resulted in a heterogeneous surface that was abundant in both hydrophobic and hydrophilic functional groups. SMX and ENR adsorption were best described using a pseudo-second-order rate expression. The SMX and ENR adsorption equilibrium data on cLND450 and cLND550 revealed their better compliance with a Langmuir isotherm than with four other models based on 2.3-fold higher values of q

Identifiants

pubmed: 36140040
pii: antibiotics11091261
doi: 10.3390/antibiotics11091261
pmc: PMC9495318
pii:
doi:

Types de publication

Journal Article

Langues

eng

Subventions

Organisme : The Office of the Ministry of Higher Education, Science, Research and Innovation; and the Thailand Science Research and Innovation through the Kasetsart University Reinventing University Program 2021.
ID : KU Reinventing program 2021

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Auteurs

Chanat Chokejaroenrat (C)

Department of Environmental Technology and Management, Faculty of Environment, Kasetsart University, Bangkok 10900, Thailand.

Chainarong Sakulthaew (C)

Department of Veterinary Technology, Faculty of Veterinary Technology, Kasetsart University, Bangkok 10900, Thailand.

Khomson Satchasataporn (K)

Department of Veterinary Technology, Faculty of Veterinary Technology, Kasetsart University, Bangkok 10900, Thailand.

Daniel D Snow (DD)

Water Sciences Laboratory, Nebraska Water Center/School of Natural Resources, University of Nebraska-Lincoln, Lincoln, NE 68583-0844, USA.

Tarik E Ali (TE)

Department of Chemistry, Faculty of Science, King Khalid University, Abha 62529, Saudi Arabia.
Department of Chemistry, Faculty of Education, Ain Shams University, Cairo 11566, Egypt.

Mohammed A Assiri (MA)

Department of Chemistry, Faculty of Science, King Khalid University, Abha 62529, Saudi Arabia.

Apichon Watcharenwong (A)

School of Environmental Engineering, Institute of Engineering, Suranaree University of Technology, Nakhon Ratchasima 30000, Thailand.
Center of Excellence in Advanced Functional Materials, Suranaree University of Technology, Nakhon Ratchasima 30000, Thailand.

Saksit Imman (S)

Integrated Biorefinery Excellent Center (IBC), School of Energy and Environment, University of Phayao, Tambon Maeka, Amphur Muang, Phayao 56000, Thailand.

Nopparat Suriyachai (N)

Integrated Biorefinery Excellent Center (IBC), School of Energy and Environment, University of Phayao, Tambon Maeka, Amphur Muang, Phayao 56000, Thailand.

Torpong Kreetachat (T)

Integrated Biorefinery Excellent Center (IBC), School of Energy and Environment, University of Phayao, Tambon Maeka, Amphur Muang, Phayao 56000, Thailand.

Classifications MeSH