Kondo quasiparticle dynamics observed by resonant inelastic x-ray scattering.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
17 Oct 2022
Historique:
received: 10 01 2022
accepted: 15 09 2022
entrez: 17 10 2022
pubmed: 18 10 2022
medline: 18 10 2022
Statut: epublish

Résumé

Effective models focused on pertinent low-energy degrees of freedom have substantially contributed to our qualitative understanding of quantum materials. An iconic example, the Kondo model, was key to demonstrating that the rich phase diagrams of correlated metals originate from the interplay of localized and itinerant electrons. Modern electronic structure calculations suggest that to achieve quantitative material-specific models, accurate consideration of the crystal field and spin-orbit interactions is imperative. This poses the question of how local high-energy degrees of freedom become incorporated into a collective electronic state. Here, we use resonant inelastic x-ray scattering (RIXS) on CePd

Identifiants

pubmed: 36253344
doi: 10.1038/s41467-022-33468-6
pii: 10.1038/s41467-022-33468-6
pmc: PMC9576770
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

6129

Subventions

Organisme : U.S. Department of Energy (DOE)
ID : DE-AC02-05CH11231
Organisme : EC | EU Framework Programme for Research and Innovation H2020 | H2020 Priority Excellent Science | H2020 European Research Council (H2020 Excellent Science - European Research Council)
ID : 646807-EXMAG
Organisme : MEXT | Japan Society for the Promotion of Science (JSPS)
ID : 21K13884
Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : SE1441/5-2
Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : CRC 1143
Organisme : EC | EC Seventh Framework Programm | FP7 Ideas: European Research Council (FP7-IDEAS-ERC - Specific Programme: "Ideas" Implementing the Seventh Framework Programme of the European Community for Research, Technological Development and Demonstration Activities (2007 to 2013))
ID : 291763

Informations de copyright

© 2022. The Author(s).

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Auteurs

M C Rahn (MC)

Los Alamos National Laboratory, Los Alamos, NM, 87545, USA. marein.rahn@tu-dresden.de.
Institute for Solid State and Materials Physics, Technical University of Dresden, 01062, Dresden, Germany. marein.rahn@tu-dresden.de.

K Kummer (K)

European Synchrotron Radiation Facility, BP 220, F-38043, Grenoble Cedex, France.

A Hariki (A)

Department of Physics and Electronics, Graduate School of Engineering, Osaka Prefecture University, Sakai, Osaka, 599-8531, Japan.
Institute for Solid State Physics, TU Wien, 1040, Vienna, Austria.

K-H Ahn (KH)

Institute for Solid State Physics, TU Wien, 1040, Vienna, Austria.
Institute of Physics of the CAS, Cukrovarnická 10, 162 00, Praha 6, Czechia.

J Kuneš (J)

Institute for Solid State Physics, TU Wien, 1040, Vienna, Austria.

A Amorese (A)

Institute of Physics II, University of Cologne, Cologne, Germany.
Max Planck Institute for Chemical Physics of Solids, Dresden, Germany.

J D Denlinger (JD)

Advanced Light Source, Lawrence Berkeley Laboratory, Berkeley, CA, 94720, USA.

D-H Lu (DH)

Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA, 94025, USA.

M Hashimoto (M)

Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA, 94025, USA.

E Rienks (E)

Helmholtz Zentrum Berlin, Bessy II, D-12489, Berlin, Germany.

M Valvidares (M)

ALBA Synchrotron Light Source, E-08290, Cerdanyola del Vallès, Barcelona, Spain.

F Haslbeck (F)

Physik-Department, Technische Universität München, D-85748, Garching, Germany.
Institute for Advanced Studies, Technische Universität München, D-85748, Garching, Germany.

D D Byler (DD)

Los Alamos National Laboratory, Los Alamos, NM, 87545, USA.

K J McClellan (KJ)

Los Alamos National Laboratory, Los Alamos, NM, 87545, USA.

E D Bauer (ED)

Los Alamos National Laboratory, Los Alamos, NM, 87545, USA.

J X Zhu (JX)

Los Alamos National Laboratory, Los Alamos, NM, 87545, USA.

C H Booth (CH)

Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

A D Christianson (AD)

Oak Ridge National Laboratory, Oak Ridge, TN, 37831, USA.

J M Lawrence (JM)

Los Alamos National Laboratory, Los Alamos, NM, 87545, USA.
Department of Physics and Astronomy, University of California, Irvine, CA, 92697, USA.

F Ronning (F)

Los Alamos National Laboratory, Los Alamos, NM, 87545, USA.

M Janoschek (M)

Los Alamos National Laboratory, Los Alamos, NM, 87545, USA. marc.janoschek@psi.ch.
Institute for Advanced Studies, Technische Universität München, D-85748, Garching, Germany. marc.janoschek@psi.ch.
Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA. marc.janoschek@psi.ch.
Laboratory for Neutron and Muon Instrumentation, Paul Scherrer Institute, CH-5232, Villigen, Switzerland. marc.janoschek@psi.ch.
Physik-Institut, Universität Zürich, Winterthurerstrasse 190, CH-8057, Zürich, Switzerland. marc.janoschek@psi.ch.

Classifications MeSH