Trypanocidal and cell swelling activity of 20-deoxysalinomycin.

20-Deoxysalinomycin African trypanosomiasis Polyether ionophores Trypanosoma brucei

Journal

Experimental parasitology
ISSN: 1090-2449
Titre abrégé: Exp Parasitol
Pays: United States
ID NLM: 0370713

Informations de publication

Date de publication:
Dec 2022
Historique:
received: 05 09 2022
revised: 12 10 2022
accepted: 18 10 2022
pubmed: 24 10 2022
medline: 30 11 2022
entrez: 23 10 2022
Statut: ppublish

Résumé

The naturally occurring polyether ionophore salinomycin was previously found to display promising anti-proliferative activity against bloodstream forms of Trypanosoma brucei. Here, we report the evaluation of 20-deoxysalinomycin, a naturally occurring homolog to salinomycin, for trypanocidal and cell swelling activity. The concentration of 20-deoxysalinomycin required to reduce the growth rate of bloodstream-form trypanosomes by 50% was determined to be 0.12 μM and found to be 8 times more trypanocidal than that of salinomycin. Moreover, 20-deoxysalinomycin and salinomycin displayed similar cytotoxic activity against human HL-60 cells. Measured as the ratio of cytotoxic to trypanocidal activity, 20-deoxysalinomycin thus exhibits a four-fold higher selectivity compared to salinomycin. The stronger trypanocidal activity of 20-deoxysalinomycin is attributed to an enhanced ability to induce cell swelling in trypanosomes. The findings support 20-deoxysalinomycin as a useful lead in the rational development of new and improved anti-trypanosomal drugs.

Identifiants

pubmed: 36273616
pii: S0014-4894(22)00208-9
doi: 10.1016/j.exppara.2022.108414
pii:
doi:

Substances chimiques

Trypanocidal Agents 0
20-deoxysalinomycin 64003-50-5

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

108414

Informations de copyright

Copyright © 2022 The Authors. Published by Elsevier Inc. All rights reserved.

Auteurs

Dietmar Steverding (D)

Bob Champion Research & Education Building, Norwich Medical School, University of East Anglia, Norwich, UK. Electronic address: d.steverding@uea.ac.uk.

Daniel Strand (D)

Centre for Analysis and Synthesis, Department of Chemistry, Lund University, Lund, Sweden.

Adam Huczyński (A)

Department of Medical Chemistry, Faculty of Chemistry, Adam Mickiewicz University, Poznań, Poland.

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Classifications MeSH