The Winner Takes It All: Carbon Supersedes Hexagonal Boron Nitride with Graphene on Transition Metals at High Temperatures.

2D materials adsorption energy carbon graphene hexagonal boron nitride pyrolysis

Journal

Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338

Informations de publication

Date de publication:
Dec 2022
Historique:
revised: 26 09 2022
received: 23 08 2022
pubmed: 2 11 2022
medline: 2 11 2022
entrez: 1 11 2022
Statut: ppublish

Résumé

The production of high-quality hexagonal boron nitride (h-BN) is essential for the ultimate performance of 2D materials-based devices, since it is the key 2D encapsulation material. Here, a decisive guideline is reported for fabricating high-quality h-BN on transition metals. It is crucial to exclude carbon from the h-BN related process, otherwise carbon prevails over boron and nitrogen due to its larger binding energy, thereupon forming graphene on metals after high-temperature annealing. The surface reaction-assisted conversion from h-BN to graphene with high-temperature treatments is demonstrated. The pyrolysis temperature T

Identifiants

pubmed: 36319466
doi: 10.1002/smll.202205184
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2205184

Subventions

Organisme : Horizon 2020 Framework Programme Graphene Flagship Core 3
ID : 881603
Organisme : Foundation for Research in Science and the Humanities
ID : FK-21-116

Informations de copyright

© 2022 Wiley-VCH GmbH.

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Auteurs

Adrian Hemmi (A)

Physik-Institut, Universität Zürich, Zürich, 8057, Switzerland.

Ari Paavo Seitsonen (AP)

Département de Chimie, École Normale Supérieure, Paris, F-75005, France.

Thomas Greber (T)

Physik-Institut, Universität Zürich, Zürich, 8057, Switzerland.

Huanyao Cun (H)

Physik-Institut, Universität Zürich, Zürich, 8057, Switzerland.

Classifications MeSH