Antidepressant and Neuroprotective Effects of 3-Hydroxy Paroxetine, an Analog of Paroxetine in Rats.


Journal

The international journal of neuropsychopharmacology
ISSN: 1469-5111
Titre abrégé: Int J Neuropsychopharmacol
Pays: England
ID NLM: 9815893

Informations de publication

Date de publication:
22 03 2023
Historique:
received: 06 09 2022
accepted: 21 11 2022
pubmed: 27 11 2022
medline: 25 3 2023
entrez: 26 11 2022
Statut: ppublish

Résumé

Paroxetine (PX) is a widely used antidepressant with side effects such as weakness, dizziness, and trouble sleeping. In search of novel compounds with better efficacy and fewer side effects, we synthesized 3HPX, a hydroxylated analog of PX, and compared the 2 in silico for their pharmacokinetic and binding properties and in vivo for their antidepressant and potential neuroprotective effects. In silico studies compared pharmacological properties as well as interactions of PX and 3HPX with the serotonin transporter. In vivo studies utilized an animal model of comorbid depression-Parkinson disease. Adult male Wistar rats were injected (sterotaxically) with lipopolysaccharide in the striatum (unilaterally), followed by 14 days of once-daily injections (i.p.) of 10 mg/kg PX or 3HPX. Animals were tested for motor asymmetry and locomotor activity as well as indices of anhedonia and helplessness using sucrose preference and forced swim tests, respectively. Brains of these animals were collected after the last test, and tyrosine hydroxylase-positive neurons in substantia nigra pars compacta and Iba-1-positive stained microglia in ipsilateral striatum were measured. In silico findings indicated that 3HPX could bind stronger to serotonin transporter and also have a better clearance and hence less toxicity compared with PX. In vivo results revealed a more effective reversal of immobility in the swim test, substantial increase in tyrosine hydroxylase-positive cells in the substantia nigra pars compacta, and more ramified Iba-1+ cells by 3HPX compared with PX. The findings suggest superior effectiveness of 3HPX as an antidepressant and neuroprotectant compared with PX and hence potential utility in Parkinson disease depression co-morbidity.

Sections du résumé

BACKGROUND
Paroxetine (PX) is a widely used antidepressant with side effects such as weakness, dizziness, and trouble sleeping. In search of novel compounds with better efficacy and fewer side effects, we synthesized 3HPX, a hydroxylated analog of PX, and compared the 2 in silico for their pharmacokinetic and binding properties and in vivo for their antidepressant and potential neuroprotective effects.
METHODS
In silico studies compared pharmacological properties as well as interactions of PX and 3HPX with the serotonin transporter. In vivo studies utilized an animal model of comorbid depression-Parkinson disease. Adult male Wistar rats were injected (sterotaxically) with lipopolysaccharide in the striatum (unilaterally), followed by 14 days of once-daily injections (i.p.) of 10 mg/kg PX or 3HPX. Animals were tested for motor asymmetry and locomotor activity as well as indices of anhedonia and helplessness using sucrose preference and forced swim tests, respectively. Brains of these animals were collected after the last test, and tyrosine hydroxylase-positive neurons in substantia nigra pars compacta and Iba-1-positive stained microglia in ipsilateral striatum were measured.
RESULTS
In silico findings indicated that 3HPX could bind stronger to serotonin transporter and also have a better clearance and hence less toxicity compared with PX. In vivo results revealed a more effective reversal of immobility in the swim test, substantial increase in tyrosine hydroxylase-positive cells in the substantia nigra pars compacta, and more ramified Iba-1+ cells by 3HPX compared with PX.
CONCLUSION
The findings suggest superior effectiveness of 3HPX as an antidepressant and neuroprotectant compared with PX and hence potential utility in Parkinson disease depression co-morbidity.

Identifiants

pubmed: 36433759
pii: 6847545
doi: 10.1093/ijnp/pyac077
pmc: PMC10032298
doi:

Substances chimiques

Paroxetine 41VRH5220H
Neuroprotective Agents 0
Tyrosine 3-Monooxygenase EC 1.14.16.2
Serotonin Plasma Membrane Transport Proteins 0
Antidepressive Agents 0

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

230-239

Informations de copyright

© The Author(s) 2022. Published by Oxford University Press on behalf of CINP.

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Auteurs

Pedro Efraín Hernández-Arrambide (PE)

Laboratorio de Neuroquímica, Facultad de Ciencias Químicas Benemérita Universidad Autónoma de Puebla, Puebla, Mexico.

Alan Carrasco-Carballo (A)

Laboratorio de Elucidación y Síntesis en Química Orgánica, Facultad de Ciencias Químicas, Benemérita Universidad Autónoma de Puebla, Puebla, Mexico.

Irving Parra (I)

Laboratorio de Neuroquímica, Facultad de Ciencias Químicas Benemérita Universidad Autónoma de Puebla, Puebla, Mexico.

Delfino Chamorro-Arenas (D)

Laboratorio de Síntesis Orgánica, Facultad de Ciencias Químicas, Benemérita Universidad Autónoma de Puebla, Puebla, Mexico.

Isabel Martínez (I)

Laboratorio de Neuroquímica, Facultad de Ciencias Químicas Benemérita Universidad Autónoma de Puebla, Puebla, Mexico.

Félix Luna (F)

Laboratorio de Neuroendocrinología, Facultad de Ciencias Químicas, Benemérita Universidad Autónoma de Puebla, Puebla, Mexico.

Fernando Sartillo-Piscil (F)

Laboratorio de Síntesis Orgánica, Facultad de Ciencias Químicas, Benemérita Universidad Autónoma de Puebla, Puebla, Mexico.

Yousef Tizabi (Y)

Department of Pharmacology, Howard University College of Medicine, Washington DC, USA.

Liliana Mendieta (L)

Laboratorio de Neuroquímica, Facultad de Ciencias Químicas Benemérita Universidad Autónoma de Puebla, Puebla, Mexico.

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Classifications MeSH