Analysis of the ability of vitamin D3-metabolizing cytochromes P450 to act on vitamin D3 sulfate and 25-hydroxyvitamin D3 3-sulfate.


Journal

The Journal of steroid biochemistry and molecular biology
ISSN: 1879-1220
Titre abrégé: J Steroid Biochem Mol Biol
Pays: England
ID NLM: 9015483

Informations de publication

Date de publication:
03 2023
Historique:
received: 08 09 2022
revised: 08 11 2022
accepted: 25 11 2022
pubmed: 2 12 2022
medline: 8 2 2023
entrez: 1 12 2022
Statut: ppublish

Résumé

25-Hydroxyvitamin D3 (25(OH)D3) is present in the human circulation esterified to sulfate with some studies showing that 25(OH)D3 3-sulfate levels are almost as high as unconjugated 25(OH)D3. Vitamin D3 is also present in human serum in the sulfated form as are other metabolites. Our aim was to determine whether sulfated forms of vitamin D3 and vitamin D3 metabolites can be acted on by vitamin D-metabolizing cytochromes P450 (CYPs), one of which (CYP11A1) is known to act on cholesterol sulfate. We used purified, bacterially expressed CYPs to test if they could act on the sulfated forms of their natural substrates. Purified CYP27A1 converted vitamin D3 sulfate to 25(OH)D3 3-sulfate with a catalytic efficiency (k

Identifiants

pubmed: 36455719
pii: S0960-0760(22)00180-7
doi: 10.1016/j.jsbmb.2022.106229
pii:
doi:

Substances chimiques

vitamin D3 sulfoconjugate 10529-43-8
Calcifediol P6YZ13C99Q
Cholesterol Side-Chain Cleavage Enzyme EC 1.14.15.6
Sulfates 0
Cholecalciferol 1C6V77QF41
Vitamin D 1406-16-2
25-Hydroxyvitamin D3 1-alpha-Hydroxylase EC 1.14.15.18
Vitamin D3 24-Hydroxylase EC 1.14.15.16
Cholestanetriol 26-Monooxygenase EC 1.14.15.15

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

106229

Informations de copyright

Copyright © 2022 Elsevier Ltd. All rights reserved.

Déclaration de conflit d'intérêts

Conflict of interest The authors declare no conflict of interest.

Auteurs

Robert C Tuckey (RC)

School of Molecular Sciences, The University of Western Australia, Perth, WA 6009, Australia. Electronic address: robert.tuckey@uwa.edu.au.

Chloe Y S Cheng (CYS)

School of Molecular Sciences, The University of Western Australia, Perth, WA 6009, Australia.

Lei Li (L)

School of Molecular Sciences, The University of Western Australia, Perth, WA 6009, Australia.

Yuhan Jiang (Y)

School of Molecular Sciences, The University of Western Australia, Perth, WA 6009, Australia.

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Classifications MeSH