Emergence of Spinons in Layered Trimer Iridate Ba_{4}Ir_{3}O_{10}.


Journal

Physical review letters
ISSN: 1079-7114
Titre abrégé: Phys Rev Lett
Pays: United States
ID NLM: 0401141

Informations de publication

Date de publication:
11 Nov 2022
Historique:
received: 04 01 2022
accepted: 17 10 2022
entrez: 3 12 2022
pubmed: 4 12 2022
medline: 4 12 2022
Statut: ppublish

Résumé

Spinons are well known as the elementary excitations of one-dimensional antiferromagnetic chains, but means to realize spinons in higher dimensions is the subject of intense research. Here, we use resonant x-ray scattering to study the layered trimer iridate Ba_{4}Ir_{3}O_{10}, which shows no magnetic order down to 0.2 K. An emergent one-dimensional spinon continuum is observed that can be well described by XXZ spin-1/2 chains with a magnetic exchange of ∼55  meV and a small Ising-like anisotropy. With 2% isovalent Sr doping, magnetic order appears below T_{N}=130  K along with sharper excitations in (Ba_{1-x}Sr_{x})_{4}Ir_{3}O_{10}. Combining our data with exact diagonalization calculations, we find that the frustrated intratrimer interactions effectively reduce the system into decoupled spin chains, the subtle balance of which can be easily tipped by perturbations such as chemical doping. Our results put Ba_{4}Ir_{3}O_{10} between the one-dimensional chain and two-dimensional quantum spin liquid scenarios, illustrating a new way to suppress magnetic order and realize fractional spinons.

Identifiants

pubmed: 36461990
doi: 10.1103/PhysRevLett.129.207201
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

207201

Auteurs

Y Shen (Y)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA.

J Sears (J)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA.

G Fabbris (G)

Advanced Photon Source, Argonne National Laboratory, Argonne, Illinois 60439, USA.

A Weichselbaum (A)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA.

W Yin (W)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA.

H Zhao (H)

Department of Physics, University of Colorado Boulder, Boulder, Colorado 80309, USA.

D G Mazzone (DG)

Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institut, CH-5232 Villigen, Switzerland.

H Miao (H)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA.
Material Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, USA.

M H Upton (MH)

Advanced Photon Source, Argonne National Laboratory, Argonne, Illinois 60439, USA.

D Casa (D)

Advanced Photon Source, Argonne National Laboratory, Argonne, Illinois 60439, USA.

R Acevedo-Esteves (R)

National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, New York 11973, USA.

C Nelson (C)

National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, New York 11973, USA.

A M Barbour (AM)

National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, New York 11973, USA.

C Mazzoli (C)

National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, New York 11973, USA.

G Cao (G)

Department of Physics, University of Colorado Boulder, Boulder, Colorado 80309, USA.

M P M Dean (MPM)

Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA.

Classifications MeSH