Discovery of High-Entropy Oxide Electrocatalysts: From Thin-Film Material Libraries to Particles.
Journal
Chemistry of materials : a publication of the American Chemical Society
ISSN: 0897-4756
Titre abrégé: Chem Mater
Pays: United States
ID NLM: 9884133
Informations de publication
Date de publication:
13 Dec 2022
13 Dec 2022
Historique:
received:
14
05
2022
revised:
02
11
2022
entrez:
19
12
2022
pubmed:
20
12
2022
medline:
20
12
2022
Statut:
ppublish
Résumé
Discovery of new high-entropy electrocatalysts requires testing of hundreds to thousands of possible compositions, which can be addressed most efficiently by high-throughput experimentation on thin-film material libraries. Since the conditions for high-throughput measurements ("screening") differ from more standardized methods, it is frequently a concern whether the findings from screening can be transferred to the commonly used particulate catalysts. We demonstrate the successful transfer of results from thin-film material libraries to particles of Cantor alloy oxide (Co-Cr-Fe-Mn-Ni)
Identifiants
pubmed: 36530940
doi: 10.1021/acs.chemmater.2c01455
pmc: PMC9753560
doi:
Types de publication
Journal Article
Langues
eng
Pagination
10291-10303Informations de copyright
© 2022 American Chemical Society.
Déclaration de conflit d'intérêts
The authors declare no competing financial interest.
Références
Angew Chem Int Ed Engl. 2020 Mar 27;59(14):5844-5850
pubmed: 31867829
ChemSusChem. 2015 Apr 13;8(7):1270-8
pubmed: 25727402
Chem Sci. 2017 Jul 1;8(7):4779-4794
pubmed: 29163926
Nat Commun. 2015 Sep 29;6:8485
pubmed: 26415623
Sci Adv. 2021 May 12;7(20):
pubmed: 33980494
ACS Nano. 2019 Oct 22;13(10):11469-11476
pubmed: 31545026
ChemSusChem. 2020 Apr 21;13(8):2038-2042
pubmed: 31981404
Adv Mater. 2019 Oct;31(41):e1902509
pubmed: 31361056
Angew Chem Int Ed Engl. 2021 Nov 2;60(45):24144-24152
pubmed: 34506069
Nanoscale. 2021 Aug 14;13(30):12788-12817
pubmed: 34477767
Angew Chem Int Ed Engl. 2021 Dec 20;60(52):26894-26903
pubmed: 34436810
Sci Rep. 2016 May 17;6:25771
pubmed: 27185646
Chem Soc Rev. 2019 Jun 17;48(12):3181-3192
pubmed: 31112142
Adv Mater. 2021 Jun;33(22):e2100745
pubmed: 33876867
Small Methods. 2021 Jan;5(1):e2000719
pubmed: 34927809
Chempluschem. 2020 Feb;85(2):327-333
pubmed: 32048799
Phys Chem Chem Phys. 2018 Nov 28;20(46):29452-29461
pubmed: 30456399
Angew Chem Int Ed Engl. 2021 Mar 22;60(13):6932-6937
pubmed: 33372334
Nano Converg. 2020 Jun 8;7(1):20
pubmed: 32514813
Phys Chem Chem Phys. 2016 Apr 21;18(15):10516-27
pubmed: 27031671
J Am Chem Soc. 2020 Mar 11;142(10):4550-4554
pubmed: 32105461
iScience. 2021 Feb 12;24(3):102177
pubmed: 33718829
Science. 2018 Mar 30;359(6383):1489-1494
pubmed: 29599236
Adv Mater. 2018 Jun;30(23):e1707512
pubmed: 29687496
Nano Converg. 2021 Feb 11;8(1):4
pubmed: 33575919
Adv Mater. 2019 Mar;31(12):e1807898
pubmed: 30680800