HPMA copolymer conjugated 5-aminolevulinic acid exhibits superior efficacy for photodynamic therapy with tumor-responsive and targeting properties.


Journal

Nanomedicine : nanotechnology, biology, and medicine
ISSN: 1549-9642
Titre abrégé: Nanomedicine
Pays: United States
ID NLM: 101233142

Informations de publication

Date de publication:
02 2023
Historique:
received: 15 09 2022
revised: 21 11 2022
accepted: 13 12 2022
pubmed: 23 12 2022
medline: 15 2 2023
entrez: 22 12 2022
Statut: ppublish

Résumé

In this study, we developed a nanoformulation of 5-aminolevulinic acid (5-ALA) for tumor-targeted photodynamic therapy, in which 5-ALA was conjugated with a biocompatible polymer N-(2-hydroxypropyl)methacrylamide (HPMA) through the hydrazone bond, i.e., P-ALA. P-ALA behaves as the nano-sized molecule with an average size of 5.5 nm in aqueous solution. P-ALA shows a largely increased release rate in acidic pH than physiological pH, suggesting the rapid release profile in acidic tumor environment. P-ALA did not show apparent cytotoxicity up to 0.1 mg/ml, however, under light irradiation, remarkable cell death was induced with the IC

Identifiants

pubmed: 36549553
pii: S1549-9634(22)00122-8
doi: 10.1016/j.nano.2022.102636
pii:
doi:

Substances chimiques

Aminolevulinic Acid 88755TAZ87
Antineoplastic Agents 0
hydroxypropyl methacrylate UKW89XAX2X
Doxorubicin 80168379AG
Polymers 0

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

102636

Informations de copyright

Copyright © 2022 The Authors. Published by Elsevier Inc. All rights reserved.

Déclaration de conflit d'intérêts

Conflicts of interest The authors declare no conflict of interest.

Auteurs

Rayhanul Islam (R)

Faculty of Pharmaceutical Sciences, Sojo University, Ikeda 4-22-1, Nishi-ku, Kumamoto 860-0082, Japan. Electronic address: rayhanulislam88@gmail.com.

Kevin Kotalík (K)

Institute of Macromolecular Chemistry v.v.i., Academy of Sciences of the Czech Republic, Heyrovsky Sq. 2, 160 00 Prague 6, Czech Republic. Electronic address: kevin.kotalik@natur.cuni.cz.

Vladimír Šubr (V)

Institute of Macromolecular Chemistry v.v.i., Academy of Sciences of the Czech Republic, Heyrovsky Sq. 2, 160 00 Prague 6, Czech Republic. Electronic address: subr@imc.cas.cz.

Shanghui Gao (S)

Faculty of Pharmaceutical Sciences, Sojo University, Ikeda 4-22-1, Nishi-ku, Kumamoto 860-0082, Japan. Electronic address: gaoshanghui94@gmail.com.

Jian-Rong Zhou (JR)

Faculty of Pharmaceutical Sciences, Sojo University, Ikeda 4-22-1, Nishi-ku, Kumamoto 860-0082, Japan. Electronic address: zhoujr@ph.sojo-u.ac.jp.

Kazumi Yokomizo (K)

Faculty of Pharmaceutical Sciences, Sojo University, Ikeda 4-22-1, Nishi-ku, Kumamoto 860-0082, Japan. Electronic address: yoko0514@ph.sojo-u.ac.jp.

Tomáš Etrych (T)

Institute of Macromolecular Chemistry v.v.i., Academy of Sciences of the Czech Republic, Heyrovsky Sq. 2, 160 00 Prague 6, Czech Republic. Electronic address: etrych@imc.cas.cz.

Jun Fang (J)

Faculty of Pharmaceutical Sciences, Sojo University, Ikeda 4-22-1, Nishi-ku, Kumamoto 860-0082, Japan. Electronic address: fangjun@ph.sojo-u.ac.jp.

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Classifications MeSH