Drug/bioactive eluting chitosan composite foams for osteochondral tissue engineering.


Journal

International journal of biological macromolecules
ISSN: 1879-0003
Titre abrégé: Int J Biol Macromol
Pays: Netherlands
ID NLM: 7909578

Informations de publication

Date de publication:
28 Feb 2023
Historique:
received: 20 08 2022
revised: 19 12 2022
accepted: 25 12 2022
pubmed: 2 1 2023
medline: 4 2 2023
entrez: 1 1 2023
Statut: ppublish

Résumé

Joint defects associated with a variety of etiologies often extend deep into the subchondral bone leading to functional impairment and joint immobility, and it is a very challenging task to regenerate the bone-cartilage interface offering significant opportunities for biomaterial-based interventions to improve the quality of life of patients. Herein drug-/bioactive-loaded porous tissue scaffolds incorporating nano-hydroxyapatite (nHAp), chitosan (CS) and either hydroxypropyl methylcellulose (HPMC) or Bombyx mori silk fibroin (SF) are fabricated through freeze drying method as subchondral bone substitute. A combination of spectroscopy and microscopy (Fourier transform infrared (FTIR) spectroscopy, scanning electron microscopy (SEM), X-ray diffraction (XRD), energy dispersive X-ray (EDX), and X-ray fluorescence (XRF) were used to analyze the structure of the porous biomaterials. The compressive mechanical properties of these scaffolds are biomimetic of cancellous bone tissues and capable of releasing drugs/bioactives (exemplified with triamcinolone acetonide, TA, or transforming growth factor-β1, TGF-β1, respectively) over a period of days. Mouse preosteoblast MC3T3-E1 cells were observed to adhere and proliferate on the tissue scaffolds as confirmed by the cell attachment, live-dead assay and alamarBlue™ assay. Interestingly, RT-qPCR analysis showed that the TA downregulated inflammatory biomarkers and upregulated the bone-specific biomarkers, suggesting such tissue scaffolds have long-term potential for clinical application.

Identifiants

pubmed: 36587649
pii: S0141-8130(22)03216-0
doi: 10.1016/j.ijbiomac.2022.12.293
pii:
doi:

Substances chimiques

Chitosan 9012-76-4
Biocompatible Materials 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

561-574

Informations de copyright

Copyright © 2022 The Authors. Published by Elsevier B.V. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare no conflict of interest. Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Muhammad Samie (M)

Interdisciplinary Research Centre in Biomedical Materials, COMSATS University Islamabad, Lahore Campus, 54000, Pakistan; Department of Pharmacy, COMSATS University Islamabad, Abbottabad Campus, 22060, Pakistan; Department of Chemistry, Lancaster University, Lancaster, Lancashire LA1 4YB, United Kingdom; Materials Science Institute, Lancaster University, Lancaster, Lancashire LA1 4YW, United Kingdom; Institute of Pharmaceutical Sciences, Khyber Medical University, Peshawar, Khyber Pakhtunkhwa 25100, Pakistan. Electronic address: Muhammadsamie.ips@kmu.edu.pk.

Ather Farooq Khan (AF)

Interdisciplinary Research Centre in Biomedical Materials, COMSATS University Islamabad, Lahore Campus, 54000, Pakistan.

Saeed Ur Rahman (SU)

Institute of Basic Medical Sciences, Khyber Medical University, Peshawar, Khyber Pakhtunkhwa 25100, Pakistan.

Haffsah Iqbal (H)

Interdisciplinary Research Centre in Biomedical Materials, COMSATS University Islamabad, Lahore Campus, 54000, Pakistan.

Muhammad Arfat Yameen (MA)

Department of Pharmacy, COMSATS University Islamabad, Abbottabad Campus, 22060, Pakistan.

Aqif Anwar Chaudhry (AA)

Interdisciplinary Research Centre in Biomedical Materials, COMSATS University Islamabad, Lahore Campus, 54000, Pakistan.

Hanaa A Galeb (HA)

Department of Chemistry, Lancaster University, Lancaster, Lancashire LA1 4YB, United Kingdom; Department of Chemistry, Science and Arts College, Rabigh Campus, King Abdulaziz University, 21577 Jeddah, Saudi Arabia.

Nathan R Halcovitch (NR)

Department of Chemistry, Lancaster University, Lancaster, Lancashire LA1 4YB, United Kingdom.

John G Hardy (JG)

Department of Chemistry, Lancaster University, Lancaster, Lancashire LA1 4YB, United Kingdom; Materials Science Institute, Lancaster University, Lancaster, Lancashire LA1 4YW, United Kingdom. Electronic address: j.g.hardy@lancaster.ac.uk.

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Classifications MeSH