Ion-Selective Microporous Polymer Membranes with Hydrogen-Bond and Salt-Bridge Networks for Aqueous Organic Redox Flow Batteries.
energy storage
ion-conducting membranes
microporous polymers
redox flow batteries
Journal
Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358
Informations de publication
Date de publication:
Mar 2023
Mar 2023
Historique:
revised:
20
12
2022
received:
01
11
2022
pubmed:
13
1
2023
medline:
13
1
2023
entrez:
12
1
2023
Statut:
ppublish
Résumé
Redox flow batteries (RFBs) have great potential for long-duration grid-scale energy storage. Ion-conducting membranes are a crucial component in RFBs, allowing charge-carrying ions to transport while preventing the cross-mixing of redox couples. Commercial Nafion membranes are widely used in RFBs, but their unsatisfactory ionic and molecular selectivity, as well as high costs, limit the performance and the widespread deployment of this technology. To extend the longevity and reduce the cost of RFB systems, inexpensive ion-selective membranes that concurrently deliver low ionic resistance and high selectivity toward redox-active species are highly desired. Here, high-performance RFB membranes are fabricated from blends of carboxylate- and amidoxime-functionalized polymers of intrinsic microporosity, which exploit the beneficial properties of both polymers. The enthalpy-driven formation of cohesive interchain interactions, including hydrogen bonds and salt bridges, facilitates the microscopic miscibility of the blends, while ionizable functional groups within the sub-nanometer pores allow optimization of membrane ion-transport functions. The resulting microporous membranes demonstrate fast cation conduction with low crossover of redox-active molecular species, enabling improved power ratings and reduced capacity fade in aqueous RFBs using anthraquinone and ferrocyanide as redox couples.
Identifiants
pubmed: 36634684
doi: 10.1002/adma.202210098
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2210098Subventions
Organisme : European Research Council
Organisme : European Union's Horizon 2020
ID : 851272
Organisme : European Union's Horizon 2020
ID : ERC-StG-PE8-NanoMMES
Organisme : European Union's Horizon 2020
ID : 758370
Organisme : Engineering and Physical Sciences Research Council
ID : EP/V047078/1
Organisme : Engineering and Physical Sciences Research Council
ID : EP/W033356/1
Organisme : Engineering and Physical Sciences Research Council
ID : EP/P024807/1
Organisme : Engineering and Physical Sciences Research Council
ID : EP/R035105/1
Organisme : EPSRC
ID : CAM-IES
Organisme : EPSRC
ID : EP/P007767/1
Organisme : UK Energy Storage Research Hub
Organisme : China Scholarship Council
Organisme : Royal Society
Informations de copyright
© 2023 The Authors. Advanced Materials published by Wiley-VCH GmbH.
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