Copper Cocatalyst Modulated Radical Generation for Selective Heterogeneous Photosynthesis of α-Haloketones.


Journal

ACS catalysis
ISSN: 2155-5435
Titre abrégé: ACS Catal
Pays: United States
ID NLM: 101562209

Informations de publication

Date de publication:
06 Jan 2023
Historique:
received: 21 10 2022
revised: 23 11 2022
entrez: 16 1 2023
pubmed: 17 1 2023
medline: 17 1 2023
Statut: ppublish

Résumé

The α-haloketones are important precursors for synthetic chemistry and pharmaceutical applications; however, their production relies heavily on traditional synthetic methods via halogenation of ketones that are toxic and environmentally risky. Here, we report a heterogeneous photosynthetic strategy of α-haloketone production from aromatic olefins using copper-modified graphitic carbon nitride (Cu-C

Identifiants

pubmed: 36644650
doi: 10.1021/acscatal.2c05189
pmc: PMC9830627
doi:

Types de publication

Journal Article

Langues

eng

Pagination

248-255

Informations de copyright

© 2022 The Authors. Published by American Chemical Society.

Déclaration de conflit d'intérêts

The authors declare no competing financial interest.

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Auteurs

Feiyu Han (F)

Soochow Institute for Energy and Materials Innovations (SIEMIS), Soochow University, Suzhou, Jiangsu 215006, China.
SynCat@Beijing, Synfuels China Technology Co. Ltd., Leyuan South Street II, No.1, Huairou, Beijing 101407, China.

Dongsheng Zhang (D)

Soochow Institute for Energy and Materials Innovations (SIEMIS), Soochow University, Suzhou, Jiangsu 215006, China.
SynCat@Beijing, Synfuels China Technology Co. Ltd., Leyuan South Street II, No.1, Huairou, Beijing 101407, China.

Sofia Salli (S)

School of Chemistry, Cardiff University, Park Place, Cardiff CF10 3AT, U.K.

Jiani Ye (J)

Soochow Institute for Energy and Materials Innovations (SIEMIS), Soochow University, Suzhou, Jiangsu 215006, China.

Yongwang Li (Y)

SynCat@Beijing, Synfuels China Technology Co. Ltd., Leyuan South Street II, No.1, Huairou, Beijing 101407, China.
State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, CAS, Taiyuan 030001, China.

Federico Rosei (F)

Center for Energy, Materials and Telecommunications, Institut National de la Recherche Scientifique, 1650 Boulevard Lionel-Boulet, Varennes, Québec J3X 1P7, Canada.

Xiao-Dong Wen (XD)

SynCat@Beijing, Synfuels China Technology Co. Ltd., Leyuan South Street II, No.1, Huairou, Beijing 101407, China.
State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, CAS, Taiyuan 030001, China.

Hans Niemantsverdriet (H)

SynCat@Beijing, Synfuels China Technology Co. Ltd., Leyuan South Street II, No.1, Huairou, Beijing 101407, China.
SynCat@DIFFER, Syngaschem BV, HH Eindhoven 6336, The Netherlands.

Emma Richards (E)

School of Chemistry, Cardiff University, Park Place, Cardiff CF10 3AT, U.K.

Ren Su (R)

Soochow Institute for Energy and Materials Innovations (SIEMIS), Soochow University, Suzhou, Jiangsu 215006, China.
SynCat@Beijing, Synfuels China Technology Co. Ltd., Leyuan South Street II, No.1, Huairou, Beijing 101407, China.

Classifications MeSH