Helicate-to-tetrahedron transformation of chiral lanthanide supramolecular complexes induced by ionic radii effect and linker length.


Journal

Communications chemistry
ISSN: 2399-3669
Titre abrégé: Commun Chem
Pays: England
ID NLM: 101725670

Informations de publication

Date de publication:
05 Aug 2021
Historique:
received: 30 10 2020
accepted: 20 07 2021
entrez: 25 1 2023
pubmed: 5 8 2021
medline: 5 8 2021
Statut: epublish

Résumé

Controlled formation of desired lanthanide supramolecular complexes is challenging because of the difficulties in predicting coordination geometry, as well as a labile coordination number. Herein, we explore the effect of ionic radii and linker length on supramolecular species formation. A helicate-to-tetrahedron transformation occurred between [Ln

Identifiants

pubmed: 36697590
doi: 10.1038/s42004-021-00553-8
pii: 10.1038/s42004-021-00553-8
pmc: PMC9814731
doi:

Types de publication

Journal Article

Langues

eng

Pagination

116

Subventions

Organisme : National Natural Science Foundation of China (National Science Foundation of China)
ID : NSFC, 21875201
Organisme : RCUK | Engineering and Physical Sciences Research Council (EPSRC)
ID : EP/P025013/1

Informations de copyright

© 2021. The Author(s).

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Auteurs

King-Him Yim (KH)

State Key Laboratory of Chemical Biology and Drug Discovery, Department of Applied Biology and Chemical Technology, The Hong Kong Polytechnic University, Kowloon, Hong Kong.

Chi-Tung Yeung (CT)

State Key Laboratory of Chemical Biology and Drug Discovery, Department of Applied Biology and Chemical Technology, The Hong Kong Polytechnic University, Kowloon, Hong Kong.

Michael R Probert (MR)

Chemistry, School of Natural and Environmental Sciences, Newcastle University, Newcastle Upon Tyne, UK.

Wesley Ting Kwok Chan (WTK)

State Key Laboratory of Chemical Biology and Drug Discovery, Department of Applied Biology and Chemical Technology, The Hong Kong Polytechnic University, Kowloon, Hong Kong.

Lewis E Mackenzie (LE)

Department of Chemistry, Durham University, Durham, UK.

Robert Pal (R)

Department of Chemistry, Durham University, Durham, UK.

Wing-Tak Wong (WT)

State Key Laboratory of Chemical Biology and Drug Discovery, Department of Applied Biology and Chemical Technology, The Hong Kong Polytechnic University, Kowloon, Hong Kong. w.t.wong@polyu.edu.hk.
The Hong Kong Polytechnic University Shenzhen Research Institute, Shenzhen, PR China. w.t.wong@polyu.edu.hk.

Ga-Lai Law (GL)

State Key Laboratory of Chemical Biology and Drug Discovery, Department of Applied Biology and Chemical Technology, The Hong Kong Polytechnic University, Kowloon, Hong Kong. ga-lai.law@polyu.edu.hk.
The Hong Kong Polytechnic University Shenzhen Research Institute, Shenzhen, PR China. ga-lai.law@polyu.edu.hk.

Classifications MeSH