A localized view on molecular dissociation via electron-ion partial covariance.


Journal

Communications chemistry
ISSN: 2399-3669
Titre abrégé: Commun Chem
Pays: England
ID NLM: 101725670

Informations de publication

Date de publication:
28 Mar 2022
Historique:
received: 19 11 2021
accepted: 21 02 2022
entrez: 25 1 2023
pubmed: 26 1 2023
medline: 26 1 2023
Statut: epublish

Résumé

Inner-shell photoelectron spectroscopy provides an element-specific probe of molecular structure, as core-electron binding energies are sensitive to the chemical environment. Short-wavelength femtosecond light sources, such as Free-Electron Lasers (FELs), even enable time-resolved site-specific investigations of molecular photochemistry. Here, we study the ultraviolet photodissociation of the prototypical chiral molecule 1-iodo-2-methylbutane, probed by extreme-ultraviolet (XUV) pulses from the Free-electron LASer in Hamburg (FLASH) through the ultrafast evolution of the iodine 4d binding energy. Methodologically, we employ electron-ion partial covariance imaging as a technique to isolate otherwise elusive features in a two-dimensional photoelectron spectrum arising from different photofragmentation pathways. The experimental and theoretical results for the time-resolved electron spectra of the 4d

Identifiants

pubmed: 36697752
doi: 10.1038/s42004-022-00656-w
pii: 10.1038/s42004-022-00656-w
pmc: PMC9814695
doi:

Types de publication

Journal Article

Langues

eng

Pagination

42

Subventions

Organisme : Volkswagen Foundation (VolkswagenStiftung)
ID : 93285
Organisme : RCUK | Engineering and Physical Sciences Research Council (EPSRC)
ID : EP/L005913/1
Organisme : RCUK | Engineering and Physical Sciences Research Council (EPSRC)
ID : EP/T021675
Organisme : RCUK | Engineering and Physical Sciences Research Council (EPSRC)
ID : EP/S028617
Organisme : RCUK | Engineering and Physical Sciences Research Council (EPSRC)
ID : EP/L005913/1
Organisme : Bundesministerium für Bildung und Forschung (Federal Ministry of Education and Research)
ID : 05K10KT2
Organisme : Bundesministerium für Bildung und Forschung (Federal Ministry of Education and Research)
ID : 05K13KT2
Organisme : Bundesministerium für Bildung und Forschung (Federal Ministry of Education and Research)
ID : 05K16KT3
Organisme : Bundesministerium für Bildung und Forschung (Federal Ministry of Education and Research)
ID : 05K10KTB
Organisme : Helmholtz Association
ID : VH-NG-1104
Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : SFB 755

Informations de copyright

© 2022. The Author(s).

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Auteurs

Felix Allum (F)

The Chemistry Research Laboratory, Department of Chemistry, University of Oxford, Oxford, OX1 3TA, UK. fallum@stanford.edu.
Stanford PULSE Institute, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA, 94025, USA. fallum@stanford.edu.

Valerija Music (V)

Institut für Physik und CINSaT, Universität Kassel, Heinrich-Plett-Straße 40, D-34132, Kassel, Germany.
European XFEL, Holzkoppel 4, 22869, Schenefeld, Germany.
Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.

Ludger Inhester (L)

Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany. ludger.inhester@desy.de.

Rebecca Boll (R)

European XFEL, Holzkoppel 4, 22869, Schenefeld, Germany.

Benjamin Erk (B)

Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.

Philipp Schmidt (P)

Institut für Physik und CINSaT, Universität Kassel, Heinrich-Plett-Straße 40, D-34132, Kassel, Germany.
European XFEL, Holzkoppel 4, 22869, Schenefeld, Germany.

Thomas M Baumann (TM)

European XFEL, Holzkoppel 4, 22869, Schenefeld, Germany.

Günter Brenner (G)

Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.

Michael Burt (M)

The Chemistry Research Laboratory, Department of Chemistry, University of Oxford, Oxford, OX1 3TA, UK.

Philipp V Demekhin (PV)

Institut für Physik und CINSaT, Universität Kassel, Heinrich-Plett-Straße 40, D-34132, Kassel, Germany.

Simon Dörner (S)

Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.

Arno Ehresmann (A)

Institut für Physik und CINSaT, Universität Kassel, Heinrich-Plett-Straße 40, D-34132, Kassel, Germany.

Andreas Galler (A)

European XFEL, Holzkoppel 4, 22869, Schenefeld, Germany.

Patrik Grychtol (P)

European XFEL, Holzkoppel 4, 22869, Schenefeld, Germany.

David Heathcote (D)

The Chemistry Research Laboratory, Department of Chemistry, University of Oxford, Oxford, OX1 3TA, UK.

Denis Kargin (D)

Institut für Chemie, Universität Kassel, Heinrich-Plett-Straße 40, D-34132, Kassel, Germany.

Mats Larsson (M)

Stockholm University, AlbaNova University Center, 114 21, Stockholm, Sweden.

Jason W L Lee (JWL)

The Chemistry Research Laboratory, Department of Chemistry, University of Oxford, Oxford, OX1 3TA, UK.
Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.

Zheng Li (Z)

Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.
State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing, 100871, China.

Bastian Manschwetus (B)

Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.

Lutz Marder (L)

Institut für Physik und CINSaT, Universität Kassel, Heinrich-Plett-Straße 40, D-34132, Kassel, Germany.

Robert Mason (R)

The Chemistry Research Laboratory, Department of Chemistry, University of Oxford, Oxford, OX1 3TA, UK.

Michael Meyer (M)

European XFEL, Holzkoppel 4, 22869, Schenefeld, Germany.

Huda Otto (H)

Institut für Physik und CINSaT, Universität Kassel, Heinrich-Plett-Straße 40, D-34132, Kassel, Germany.

Christopher Passow (C)

Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.

Rudolf Pietschnig (R)

Institut für Chemie, Universität Kassel, Heinrich-Plett-Straße 40, D-34132, Kassel, Germany.

Daniel Ramm (D)

Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.

Kaja Schubert (K)

Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.

Lucas Schwob (L)

Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.

Richard D Thomas (RD)

Stockholm University, AlbaNova University Center, 114 21, Stockholm, Sweden.

Claire Vallance (C)

The Chemistry Research Laboratory, Department of Chemistry, University of Oxford, Oxford, OX1 3TA, UK.

Igor Vidanović (I)

Institut für Chemie, Universität Kassel, Heinrich-Plett-Straße 40, D-34132, Kassel, Germany.

Clemens von Korff Schmising (C)

Max Born Institute, Max-Born-Straße 2A, 12489, Berlin, Germany.

René Wagner (R)

European XFEL, Holzkoppel 4, 22869, Schenefeld, Germany.

Peter Walter (P)

SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA, 94025, USA.

Vitali Zhaunerchyk (V)

University of Gothenburg, 405 30, Gothenburg, Sweden.

Daniel Rolles (D)

J. R. Macdonald Laboratory, Physics Department, Kansas State University, 1228 Martin Luther King Jr. Dr., Manhattan, KS, 66506, USA.

Sadia Bari (S)

Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.

Mark Brouard (M)

The Chemistry Research Laboratory, Department of Chemistry, University of Oxford, Oxford, OX1 3TA, UK.

Markus Ilchen (M)

Institut für Physik und CINSaT, Universität Kassel, Heinrich-Plett-Straße 40, D-34132, Kassel, Germany. markus.ilchen@desy.de.
European XFEL, Holzkoppel 4, 22869, Schenefeld, Germany. markus.ilchen@desy.de.
Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany. markus.ilchen@desy.de.

Classifications MeSH