Structure and properties of polylactic acid/butenediol vinyl alcohol copolymer blend fibers.

Biodegradable Butenediol vinyl alcohol copolymer (BVOH) Drug release Miscibility Polylactic acid (PLA)

Journal

International journal of biological macromolecules
ISSN: 1879-0003
Titre abrégé: Int J Biol Macromol
Pays: Netherlands
ID NLM: 7909578

Informations de publication

Date de publication:
31 Mar 2023
Historique:
received: 13 11 2022
revised: 07 01 2023
accepted: 19 01 2023
pubmed: 27 1 2023
medline: 9 3 2023
entrez: 26 1 2023
Statut: ppublish

Résumé

Polylactic acid/butenediol vinyl alcohol copolymer (PLA/BVOH) blends with different weight ratios were prepared by melt mixing. PLA and BVOH in PLA/BVOH blends were immiscible while the weak interaction between PLA and BVOH existed. The introduction of BVOH facilitated the crystallization of PLA. Moreover, the crystallization of PLA hindered the crystallization of BVOH. Due to introduction of BVOH, PLA/BVOH blends exhibited shear thinning characteristic except that PLA/BVOH blends with 5-10 % BVOH showed similar rheological property to neat PLA. With the increase of BVOH content, the contact angle of PLA/BVOH blends decreased from 79.75° to 67.33° at 120 s. The hydrophilicity of PLA/BVOH blends was improved. In addition, PLA/BVOH fibers with 5-40 % BVOH and PLA/BVOH/rutin fibers with 3 % rutin were manufactured by melt spinning. The effect of BVOH on the mechanical property of PLA/BVOH fibers was small. However, BVOH improved significantly the rutin release rate and antioxidant properties of PLA/BVOH/rutin fibers.

Identifiants

pubmed: 36702218
pii: S0141-8130(23)00282-9
doi: 10.1016/j.ijbiomac.2023.123396
pii:
doi:

Substances chimiques

poly(lactide) 459TN2L5F5
Polymers 0
Polyesters 0
Ethanol 3K9958V90M
Vinyl Compounds 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

123396

Informations de copyright

Copyright © 2023 Elsevier B.V. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Dongzheng Yu (D)

Key Laboratory of Eco-Textiles, Ministry of Education, Jiangnan University, Wuxi 214122, People's Republic of China.

Qianqian Yang (Q)

Key Laboratory of Eco-Textiles, Ministry of Education, Jiangnan University, Wuxi 214122, People's Republic of China.

Xingxing Zhou (X)

Key Laboratory of Eco-Textiles, Ministry of Education, Jiangnan University, Wuxi 214122, People's Republic of China.

Haiyang Guo (H)

Jiangsu Doway New Materials Science & Technology Co. Ltd., Suqian 223800, People's Republic of China.

Dawei Li (D)

Key Laboratory of Eco-Textiles, Ministry of Education, Jiangnan University, Wuxi 214122, People's Republic of China.

Haoxuan Li (H)

Key Laboratory of Eco-Textiles, Ministry of Education, Jiangnan University, Wuxi 214122, People's Republic of China.

Bingyao Deng (B)

Key Laboratory of Eco-Textiles, Ministry of Education, Jiangnan University, Wuxi 214122, People's Republic of China.

Qingsheng Liu (Q)

Key Laboratory of Eco-Textiles, Ministry of Education, Jiangnan University, Wuxi 214122, People's Republic of China. Electronic address: qsliu@jiangnan.edu.cn.

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Classifications MeSH