Water as a Modifier in a Hybrid Coordination Network Glass.

coordination networks glass modifiers hybrid glasses melting water

Journal

Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338

Informations de publication

Date de publication:
Apr 2023
Historique:
revised: 21 12 2022
received: 29 09 2022
medline: 28 1 2023
pubmed: 28 1 2023
entrez: 27 1 2023
Statut: ppublish

Résumé

Chemical diversification of hybrid organic-inorganic glasses remains limited, especially compared to traditional oxide glasses, for which property tuning is possible through addition of weakly bonded modifier cations. In this work, it is shown that water can depolymerize polyhedra with labile metal-ligand bonds in a cobalt-based coordination network, yielding a series of nonstoichiometric glasses. Calorimetric, spectroscopic, and simulation studies demonstrate that the added water molecules promote the breakage of network bonds and coordination number changes, leading to lower melting and glass transition temperatures. These structural changes modify the physical and chemical properties of the melt-quenched glass, with strong parallels to the "modifier" concept in oxides. It is shown that this approach also applies to other transition metal-based coordination networks, and it will thus enable diversification of hybrid glass chemistry, including nonstoichiometric glass compositions, tuning of properties, and a significant rise in the number of glass-forming hybrid systems by allowing them to melt before thermal decomposition.

Identifiants

pubmed: 36703506
doi: 10.1002/smll.202205988
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2205988

Subventions

Organisme : the Independent Research Fund Denmark
ID : 0136-00011
Organisme : China Scholarship Council
ID : 201906250152
Organisme : European Union's Horizon 2020 research and innovation programme
ID : 101018156
Organisme : EuroHPC for computing resources on the Vega HPC
ID : EU2010PA6249
Organisme : National Research Foundation, Singapore
Organisme : National Science Foundation
ID : DMR-1928538
Organisme : National Science Foundation
ID : DMR-1944510

Informations de copyright

© 2023 The Authors. Small published by Wiley-VCH GmbH.

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Auteurs

Søren S Sørensen (SS)

Department of Chemistry and Bioscience, Aalborg University, Aalborg, 9220, Denmark.

Xiangting Ren (X)

Department of Chemistry and Bioscience, Aalborg University, Aalborg, 9220, Denmark.

Tao Du (T)

Department of Chemistry and Bioscience, Aalborg University, Aalborg, 9220, Denmark.

Ayoub Traverson (A)

Department of Chemistry and Bioscience, Aalborg University, Aalborg, 9220, Denmark.
Chemistry DER, University Paris-Saclay, ENS Paris-Saclay, Gif-Sur-Yvette, 91190, France.

Shibo Xi (S)

Institute of Chemical & Engineering Sciences, Technology and Research (A*STAR), Singapore, 627833, Singapore.

Lars R Jensen (LR)

Department of Materials and Production, Aalborg University, Aalborg, 9220, Denmark.

Mathieu Bauchy (M)

Department of Civil and Environmental Engineering, University of California, Los Angeles, CA, 90095, USA.

Satoshi Horike (S)

Institute for Integrated Cell-Material Sciences, Institute for Advanced Study, Kyoto University, Kyoto, 606-8501, Japan.

John Wang (J)

Department of Materials Science and Engineering, National University of Singapore, Singapore, 117574, Singapore.

Morten M Smedskjaer (MM)

Department of Chemistry and Bioscience, Aalborg University, Aalborg, 9220, Denmark.

Classifications MeSH