Detecting and Characterizing Particulate Organic Nitrates with an Aerodyne Long-ToF Aerosol Mass Spectrometer.


Journal

ACS earth & space chemistry
ISSN: 2472-3452
Titre abrégé: ACS Earth Space Chem
Pays: United States
ID NLM: 101695267

Informations de publication

Date de publication:
19 Jan 2023
Historique:
received: 13 10 2022
revised: 13 12 2022
accepted: 13 12 2022
entrez: 27 1 2023
pubmed: 28 1 2023
medline: 28 1 2023
Statut: epublish

Résumé

Particulate organic nitrate (pON) can be a major part of secondary organic aerosol (SOA) and is commonly quantified by indirect means from aerosol mass spectrometer (AMS) data. However, pON quantification remains challenging. Here, we set out to quantify and characterize pON in the boreal forest, through direct field observations at Station for Measuring Ecosystem Atmosphere Relationships (SMEAR) II in Hyytiälä, Finland, and targeted single-precursor laboratory studies. We utilized a long time-of-flight AMS (LToF-AMS) for aerosol chemical characterization, with a particular focus to identify C

Identifiants

pubmed: 36704177
doi: 10.1021/acsearthspacechem.2c00314
pmc: PMC9869397
doi:

Types de publication

Journal Article

Langues

eng

Pagination

230-242

Informations de copyright

© 2022 The Authors. Published by American Chemical Society.

Déclaration de conflit d'intérêts

The authors declare the following competing financial interest(s): A.L. and L.R.W. are employees at Aerodyne Research Inc., which manufactures the LToF-AMS and the PAM-OFR.

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Auteurs

Frans Graeffe (F)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki00014, Finland.

Liine Heikkinen (L)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki00014, Finland.
Department of Environmental Science and Bolin Centre for Climate Research, Stockholm University, StockholmSE-10691, Sweden.

Olga Garmash (O)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki00014, Finland.
Aerosol Physics Laboratory, Physics Unit, Tampere University, Tampere33014, Finland.

Mikko Äijälä (M)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki00014, Finland.

James Allan (J)

Department of Earth and Environmental Sciences and National Centre for Atmospheric Science (NCAS), University of Manchester, Oxford Road, ManchesterM13 9PL, U.K.

Anaïs Feron (A)

Univ Paris Est Créteil and Université Paris Cité, CNRS, LISA, Créteil, ParisF-94010, France.

Manuela Cirtog (M)

Univ Paris Est Créteil and Université Paris Cité, CNRS, LISA, Créteil, ParisF-94010, France.

Jean-Eudes Petit (JE)

Laboratoire des Sciences du Climat et de l'Environnement (LSCE), Gif-sur-Yvette91191, France.

Nicolas Bonnaire (N)

Laboratoire des Sciences du Climat et de l'Environnement (LSCE), Gif-sur-Yvette91191, France.

Andrew Lambe (A)

Aerodyne Research Inc., Billerica, Massachusetts01821, United States.

Olivier Favez (O)

Institut National de l'Environnement Industriel et des Risques (INERIS), Verneuil-en-Halatte60550, France.

Alexandre Albinet (A)

Institut National de l'Environnement Industriel et des Risques (INERIS), Verneuil-en-Halatte60550, France.

Leah R Williams (LR)

Aerodyne Research Inc., Billerica, Massachusetts01821, United States.

Mikael Ehn (M)

Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki00014, Finland.

Classifications MeSH