Deciphering the Role of Water in Promoting the Optoelectronic Performance of Surface-Engineered Lead Halide Perovskite Nanocrystals.

lead halide perovskites light-emitting diodes nanocrystals passivation post-treatment spectroscopy surface defects

Journal

ACS applied materials & interfaces
ISSN: 1944-8252
Titre abrégé: ACS Appl Mater Interfaces
Pays: United States
ID NLM: 101504991

Informations de publication

Date de publication:
08 Feb 2023
Historique:
pubmed: 28 1 2023
medline: 28 1 2023
entrez: 27 1 2023
Statut: ppublish

Résumé

Lead halide perovskites are promising candidates for high-performance light-emitting diodes (LEDs); however, their applicability is limited by their structural instability toward moisture. Although a deliberate addition of water to the precursor solution has recently been shown to improve the crystallinity and optical properties of perovskites, the corresponding thin films still do not exhibit a near-unity quantum yield. Herein, we report that the direct addition of a minute amount of water to post-treated formamidinium lead bromide (FAPbBr

Identifiants

pubmed: 36705637
doi: 10.1021/acsami.2c20605
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

7294-7307

Auteurs

Harshita Bhatia (H)

Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001Leuven, Belgium.

Cristina Martin (C)

Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001Leuven, Belgium.
Department of Physical Chemistry, Faculty of Pharmacy, University of Castilla-La Mancha, C/ José María Sánchez Ibañez s/n, 02071Albacete, Spain.

Masoumeh Keshavarz (M)

Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001Leuven, Belgium.

Iurii Dovgaliuk (I)

Institut des Matériaux Poreux de Paris, Ecole Normale Supérieure, ESPCI Paris, CNRS, PSL Université, 75005Paris, France.

Nadine J Schrenker (NJ)

Electron Microscopy for Materials Science (EMAT) and NANOlab Center of Excellence, University of Antwerp, Groenenborgerlaan 171, B-2020Wilrijk, Belgium.

Martin Ottesen (M)

Department of Chemistry and iNANO, Aarhus University, Langelandsgade 140, 8000Aarhus C, Denmark.

Weiming Qiu (W)

Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001Leuven, Belgium.

Eduard Fron (E)

Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001Leuven, Belgium.

Martin Bremholm (M)

Department of Chemistry and iNANO, Aarhus University, Langelandsgade 140, 8000Aarhus C, Denmark.

Joris Van de Vondel (J)

Quantum Solid-State Physics (QSP), Department of Physics and Astronomy, KU Leuven, Celestijnenlaan 200D, Leuven3001, Belgium.

Sara Bals (S)

Electron Microscopy for Materials Science (EMAT) and NANOlab Center of Excellence, University of Antwerp, Groenenborgerlaan 171, B-2020Wilrijk, Belgium.

Maarten B J Roeffaers (MBJ)

cMACS, Department of Microbial and Molecular Systems, KU Leuven, 3001Leuven, Belgium.

Johan Hofkens (J)

Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001Leuven, Belgium.

Elke Debroye (E)

Department of Chemistry, KU Leuven, Celestijnenlaan 200F, 3001Leuven, Belgium.

Classifications MeSH