Solvent Free Upgrading of 5-Hydroxymethylfurfural (HMF) with Levulinic Acid to HMF Levulinate Using Tin Exchanged Tungstophosphoric Acid Supported on K-10 Catalyst.


Journal

ACS organic & inorganic Au
ISSN: 2694-247X
Titre abrégé: ACS Org Inorg Au
Pays: United States
ID NLM: 9918282981206676

Informations de publication

Date de publication:
01 Feb 2023
Historique:
received: 09 06 2022
revised: 14 09 2022
accepted: 16 09 2022
entrez: 7 2 2023
pubmed: 8 2 2023
medline: 8 2 2023
Statut: epublish

Résumé

The manufacture of high-value products from biomass derived platform chemicals is becoming an integral part of the biorefinery industry. In this study, we demonstrate a green catalytic process using solvent free conditions for the synthesis of hydroxymethylfurfural (HMF) levulinate from HMF and levulinic acid (LA) over tin exchanged tungstophosphoric acid (DTP) supported on K-10 (montmorillonite K-10 clay) as the catalyst. The structural properties of solid acid catalysts were characterized by using XRD, FT-IR, UV-vis, titration, and SEM techniques. Partial exchange of the H

Identifiants

pubmed: 36748078
doi: 10.1021/acsorginorgau.2c00027
pmc: PMC9896477
doi:

Types de publication

Journal Article

Langues

eng

Pagination

27-34

Informations de copyright

© 2022 The Authors. Published by American Chemical Society.

Déclaration de conflit d'intérêts

The authors declare no competing financial interest.

Références

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Auteurs

Manishkumar S Tiwari (MS)

Theoretical and Applied Catalysis Research Cluster, School of Chemistry and Chemical Engineering, Queen's University Belfast, David-Keir Building, Stranmillis Road, BelfastBT9 5AG, U.K.
Department of chemical Engineering, Mukesh Patel School of Technology Management and Engineering, SVKM's NMIMS University, Mumbai, India400065.

Dipti Wagh (D)

Theoretical and Applied Catalysis Research Cluster, School of Chemistry and Chemical Engineering, Queen's University Belfast, David-Keir Building, Stranmillis Road, BelfastBT9 5AG, U.K.

Jennifer Sarah Dicks (JS)

Theoretical and Applied Catalysis Research Cluster, School of Chemistry and Chemical Engineering, Queen's University Belfast, David-Keir Building, Stranmillis Road, BelfastBT9 5AG, U.K.

John Keogh (J)

Theoretical and Applied Catalysis Research Cluster, School of Chemistry and Chemical Engineering, Queen's University Belfast, David-Keir Building, Stranmillis Road, BelfastBT9 5AG, U.K.

Michela Ansaldi (M)

Theoretical and Applied Catalysis Research Cluster, School of Chemistry and Chemical Engineering, Queen's University Belfast, David-Keir Building, Stranmillis Road, BelfastBT9 5AG, U.K.

Vivek V Ranade (VV)

Theoretical and Applied Catalysis Research Cluster, School of Chemistry and Chemical Engineering, Queen's University Belfast, David-Keir Building, Stranmillis Road, BelfastBT9 5AG, U.K.

Haresh G Manyar (HG)

Theoretical and Applied Catalysis Research Cluster, School of Chemistry and Chemical Engineering, Queen's University Belfast, David-Keir Building, Stranmillis Road, BelfastBT9 5AG, U.K.

Classifications MeSH