Dual Thermal- and Oxidation-Responsive Polymers Synthesized by a Sequential ROP-to-RAFT Procedure Inherently Temper Neuroinflammation.


Journal

Biomacromolecules
ISSN: 1526-4602
Titre abrégé: Biomacromolecules
Pays: United States
ID NLM: 100892849

Informations de publication

Date de publication:
09 10 2023
Historique:
medline: 10 10 2023
pubmed: 10 2 2023
entrez: 9 2 2023
Statut: ppublish

Résumé

This study is about multiple responsiveness in biomedical materials. This typically implies "orthogonality" (i.e., one response does not affect the other) or synergy (i.e., one increases efficacy or selectivity of the other), but an antagonist effect between responses may also occur. Here, we describe a family of very well-defined amphiphilic and micelle-forming block copolymers, which show both oxidative and temperature responses. They are produced via successive anionic ring-opening polymerization of episulfides and RAFT polymerization of dialkylacrylamides and differ only in the ratio between inert (

Identifiants

pubmed: 36757736
doi: 10.1021/acs.biomac.2c01365
pmc: PMC10565819
doi:

Substances chimiques

Polymers 0
Micelles 0
Reactive Oxygen Species 0
Anti-Inflammatory Agents 0

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

4478-4493

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Auteurs

Zulfiye Y Turhan (ZY)

Laboratory for Polymers and Biomaterials, Fondazione Istituto Italiano di Tecnologia, 16163 Genova, Italy.
Division of Pharmacy and Optometry, School of Health Sciences, University of Manchester, Oxford Road, Manchester M13 9PT, United Kingdom.

Richard d'Arcy (R)

Laboratory for Polymers and Biomaterials, Fondazione Istituto Italiano di Tecnologia, 16163 Genova, Italy.

Farah El Mohtadi (F)

Division of Pharmacy and Optometry, School of Health Sciences, University of Manchester, Oxford Road, Manchester M13 9PT, United Kingdom.

Lorena Infante Teixeira (LI)

Laboratory for Polymers and Biomaterials, Fondazione Istituto Italiano di Tecnologia, 16163 Genova, Italy.

Nora Francini (N)

Laboratory for Polymers and Biomaterials, Fondazione Istituto Italiano di Tecnologia, 16163 Genova, Italy.

Mike Geven (M)

Laboratory for Polymers and Biomaterials, Fondazione Istituto Italiano di Tecnologia, 16163 Genova, Italy.

Valentina Castagnola (V)

Center for Synaptic Neuroscience and Technology, Fondazione Istituto Italiano di Tecnologia, 16132 Genova, Italy.
IRCCS Ospedale Policlinico San Martino, 16132 Genova, Italy.

Aws Alshamsan (A)

Department of Pharmaceutics, College of Pharmacy, King Saud University, P.O. Box 2457, Riyadh 11451, Saudi Arabia.
Nanobiotechnology Unit, College of Pharmacy, King Saud University, P.O. Box 2457, Riyadh 11451, Saudi Arabia.

Fabio Benfenati (F)

Center for Synaptic Neuroscience and Technology, Fondazione Istituto Italiano di Tecnologia, 16132 Genova, Italy.
IRCCS Ospedale Policlinico San Martino, 16132 Genova, Italy.

Nicola Tirelli (N)

Laboratory for Polymers and Biomaterials, Fondazione Istituto Italiano di Tecnologia, 16163 Genova, Italy.
Division of Pharmacy and Optometry, School of Health Sciences, University of Manchester, Oxford Road, Manchester M13 9PT, United Kingdom.

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Classifications MeSH