Homogeneously Oriented Organic Single-Crystalline Patterns Grown by Microspacing In-Air Sublimation.
in-plane orientation
microspacing sublimation
organic field-effect transistor arrays
organic semiconductors
single-crystalline patterns
Journal
Small methods
ISSN: 2366-9608
Titre abrégé: Small Methods
Pays: Germany
ID NLM: 101724536
Informations de publication
Date de publication:
Apr 2023
Apr 2023
Historique:
revised:
30
11
2022
received:
24
10
2022
medline:
23
2
2023
pubmed:
23
2
2023
entrez:
22
2
2023
Statut:
ppublish
Résumé
Fabrication of single-crystalline organic semiconductor patterns is of key importance to enable practical applications. However due to the poor controllability on nucleation locations and the intrinsic anisotropic nature of single-crystals, growth of single-crystal patterns with homogeneous orientation is a big challenge especially by the vapor method. Herein a vapor growth protocol to achieve patterned organic semiconductor single-crystals with high crystallinity and uniform crystallographic orientation is presented. The protocol relies on the recently invented microspacing in-air sublimation assisted with surface wettability treatment to precisely pin the organic molecules at desired locations, and inter-connecting pattern motifs to induce homogeneous crystallographic orientation. Single-crystalline patterns with different shapes and sizes, and uniform orientation are demonstrated exemplarily by using 2,7-dioctyl[1]benzothieno[3,2-b][1]benzothiophene (C8-BTBT). Field-effect transistor arrays fabricate on the patterned C8-BTBT single-crystal patterns show uniform electrical performance: a 100% yield with an average mobility of 6.28 cm
Identifiants
pubmed: 36808831
doi: 10.1002/smtd.202201374
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2201374Subventions
Organisme : National Key Research and Development Program of China
ID : 2018YFB0406502
Organisme : 111 Project 2.0 in China
ID : PB2018013
Organisme : China Postdoctoral Science Foundation
ID : 2021M701973
Organisme : Distinguished Young Scholars of Shandong Province
ID : ZR2019JQ03
Organisme : Postdoctoral Innovation Project of Shandong Province
Organisme : Natural Science Foundation of Shandong Province
ID : ZR202105230005
Organisme : Natural Science Foundation of Shandong Province
ID : ZR2021QE091
Organisme : National Natural Science Foundation of China
ID : 52273185
Organisme : National Natural Science Foundation of China
ID : 51973106
Organisme : National Natural Science Foundation of China
ID : 52102006
Organisme : National Natural Science Foundation of China
ID : 51932004
Organisme : Qilu (Zhongying) Young Scholars
ID : nonumber
Organisme : Shandong University multidisciplinary research and innovation team of young scholars
ID : nonumber
Informations de copyright
© 2023 Wiley-VCH GmbH.
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