Non-covalent ligand-oxide interaction promotes oxygen evolution.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
22 Feb 2023
Historique:
received: 05 05 2022
accepted: 14 02 2023
entrez: 22 2 2023
pubmed: 23 2 2023
medline: 23 2 2023
Statut: epublish

Résumé

Strategies to generate high-valence metal species capable of oxidizing water often employ composition and coordination tuning of oxide-based catalysts, where strong covalent interactions with metal sites are crucial. However, it remains unexplored whether a relatively weak "non-bonding" interaction between ligands and oxides can mediate the electronic states of metal sites in oxides. Here we present an unusual non-covalent phenanthroline-CoO

Identifiants

pubmed: 36813796
doi: 10.1038/s41467-023-36718-3
pii: 10.1038/s41467-023-36718-3
pmc: PMC9947139
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

997

Subventions

Organisme : National Natural Science Foundation of China (National Science Foundation of China)
ID : 22072013

Informations de copyright

© 2023. The Author(s).

Références

Sci Rep. 2015 Jul 16;5:12167
pubmed: 26178185
J Am Chem Soc. 2015 Mar 18;137(10):3638-48
pubmed: 25700234
Nature. 2008 Jun 5;453(7196):763-6
pubmed: 18528391
Science. 2013 Apr 5;340(6128):60-3
pubmed: 23539180
Proc Natl Acad Sci U S A. 2017 Apr 11;114(15):3855-3860
pubmed: 28348217
Nat Commun. 2022 Mar 10;13(1):1243
pubmed: 35273163
Nat Mater. 2016 Dec 20;16(1):70-81
pubmed: 27994241
Nat Chem. 2012 May 06;4(6):498-502
pubmed: 22614386
J Am Chem Soc. 2013 Nov 13;135(45):16977-87
pubmed: 24171402
Nat Commun. 2017 Mar 24;8:14839
pubmed: 28337985
Phys Rev Lett. 2019 Jan 11;122(1):016805
pubmed: 31012645
Angew Chem Int Ed Engl. 2021 Jun 21;60(26):14446-14457
pubmed: 33844879
Nat Chem. 2021 Jun;13(6):523-529
pubmed: 33767362
Science. 2008 Aug 22;321(5892):1072-5
pubmed: 18669820
Nat Chem. 2018 Feb;10(2):149-154
pubmed: 29359759
Proc Natl Acad Sci U S A. 2013 Sep 24;110(39):15579-84
pubmed: 24019473
J Phys Chem Lett. 2015 Sep 17;6(18):3737-42
pubmed: 26722749
Science. 2014 Aug 15;345(6198):804-8
pubmed: 25124437
Nat Mater. 2016 Feb;15(2):121-6
pubmed: 26796721
J Am Chem Soc. 2010 May 26;132(20):6882-3
pubmed: 20433197
Nat Commun. 2019 Nov 15;10(1):5208
pubmed: 31729380
J Am Chem Soc. 2022 May 4;144(17):7622-7633
pubmed: 35442661
Science. 2010 Apr 16;328(5976):342-5
pubmed: 20223949
J Am Chem Soc. 2019 Apr 3;141(13):5231-5240
pubmed: 30860837
Proc Natl Acad Sci U S A. 2017 Feb 14;114(7):1486-1491
pubmed: 28137835
Nat Commun. 2020 Aug 13;11(1):4066
pubmed: 32792524
Nat Mater. 2021 May;20(5):674-682
pubmed: 33432142
Small. 2019 Oct;15(44):e1903847
pubmed: 31512397
J Am Chem Soc. 2016 Jun 15;138(23):7252-5
pubmed: 27232374
Angew Chem Int Ed Engl. 2006 Apr 21;45(17):2778-81
pubmed: 16548024
Nat Commun. 2014 Jun 18;5:4191
pubmed: 24939393
Angew Chem Int Ed Engl. 2018 Sep 24;57(39):12840-12844
pubmed: 30112793
Acc Chem Res. 2018 Nov 20;51(11):2968-2977
pubmed: 30375841
Nat Commun. 2020 May 20;11(1):2522
pubmed: 32433529
J Am Chem Soc. 2020 Jul 8;142(27):11901-11914
pubmed: 32539368
J Am Chem Soc. 2016 Aug 31;138(34):11017-30
pubmed: 27515121
Appl Magn Reson. 2013 Jul;44(7):817-826
pubmed: 23766555
J Synchrotron Radiat. 2005 Jul;12(Pt 4):537-41
pubmed: 15968136
J Am Chem Soc. 2017 Feb 8;139(5):1878-1884
pubmed: 28098444
J Am Chem Soc. 2011 Oct 5;133(39):15444-52
pubmed: 21913664
Nat Commun. 2017 Dec 8;8(1):2022
pubmed: 29222428
Nat Mater. 2017 Sep;16(9):925-931
pubmed: 28714982
Science. 2016 Apr 15;352(6283):333-7
pubmed: 27013427
J Am Chem Soc. 2011 Apr 13;133(14):5587-93
pubmed: 21413705

Auteurs

Qianbao Wu (Q)

Molecular Electrochemistry Laboratory, Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu, 610054, China.

Junwu Liang (J)

Optoelectronic Information Research Center, School of Physics and Telecommunication Engineering, Yulin Normal University, Yulin, Guangxi, 537000, China.

Mengjun Xiao (M)

Molecular Electrochemistry Laboratory, Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu, 610054, China.

Chang Long (C)

Molecular Electrochemistry Laboratory, Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu, 610054, China.

Lei Li (L)

Molecular Electrochemistry Laboratory, Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu, 610054, China.

Zhenhua Zeng (Z)

Davidson School of Chemical Engineering, Purdue University, West Lafayette, IN, 47907, USA. zeng46@purdue.edu.

Andraž Mavrič (A)

Materials Research Laboratory, University of Nova Gorica, Vipavska 13, SI-5000, Nova Gorica, Slovenia.

Xia Zheng (X)

Molecular Electrochemistry Laboratory, Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu, 610054, China.

Jing Zhu (J)

Department of Chemical Physics, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei, 230026, China.

Hai-Wei Liang (HW)

Hefei National Laboratory for Physical Sciences at the Microscale, Department of Chemistry, University of Science and Technology of China, Hefei, 230026, China.

Hongfei Liu (H)

Molecular Electrochemistry Laboratory, Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu, 610054, China.

Matjaz Valant (M)

Materials Research Laboratory, University of Nova Gorica, Vipavska 13, SI-5000, Nova Gorica, Slovenia.

Wei Wang (W)

School of Materials and Energy, University of Electronic Science and Technology of China, Chengdu, 610054, China.

Zhengxing Lv (Z)

Shanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai, 201210, China.

Jiong Li (J)

Shanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai, 201210, China.

Chunhua Cui (C)

Molecular Electrochemistry Laboratory, Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu, 610054, China. chunhua.cui@uestc.edu.cn.

Classifications MeSH