Theoretical study on the mechanism of water oxidation catalyzed by a mononuclear copper complex: important roles of a redox non-innocent ligand and HPO


Journal

RSC advances
ISSN: 2046-2069
Titre abrégé: RSC Adv
Pays: England
ID NLM: 101581657

Informations de publication

Date de publication:
08 Mar 2023
Historique:
received: 31 01 2023
accepted: 25 02 2023
entrez: 17 3 2023
pubmed: 18 3 2023
medline: 18 3 2023
Statut: epublish

Résumé

The water oxidation reaction is the bottleneck problem of the artificial photosynthetic system. In this work, the mechanism of water oxidation catalyzed by a mononuclear copper complex in alkaline conditions was studied by density functional calculations. Firstly, a water molecule coordinating with the copper center of the complex (Cu

Identifiants

pubmed: 36926005
doi: 10.1039/d3ra00648d
pii: d3ra00648d
pmc: PMC10011972
doi:

Types de publication

Journal Article

Langues

eng

Pagination

8352-8359

Informations de copyright

This journal is © The Royal Society of Chemistry.

Déclaration de conflit d'intérêts

The authors declare no competing financial interest.

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Auteurs

Ying-Ying Li (YY)

School of Chemistry and Chemical Engineering, Zhengzhou Normal University Zhengzhou 450044 China liyingying@zznu.edu.cn.

Xiao-Yan Wang (XY)

School of Chemistry and Chemical Engineering, Zhengzhou Normal University Zhengzhou 450044 China liyingying@zznu.edu.cn.

Hui-Ji Li (HJ)

School of Chemistry and Chemical Engineering, Zhengzhou Normal University Zhengzhou 450044 China liyingying@zznu.edu.cn.

Jia-Yi Chen (JY)

Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Bioinorganic Chemistry and Materia Medica, Hubei Key Laboratory of Materials Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology Wuhan 430074 P. R. China.

Yao-Hua Kou (YH)

School of Chemistry and Chemical Engineering, Zhengzhou Normal University Zhengzhou 450044 China liyingying@zznu.edu.cn.

Xiao Li (X)

School of Chemistry and Chemical Engineering, Zhengzhou Normal University Zhengzhou 450044 China liyingying@zznu.edu.cn.

Yaping Wang (Y)

School of Chemistry and Chemical Engineering, Zhengzhou Normal University Zhengzhou 450044 China liyingying@zznu.edu.cn.

Classifications MeSH