In Situ Detecting Thermal Stability of Solid Electrolyte Interphase (SEI).
in situ heating X-ray photoelectron spectroscopy (XPS)
lithium-ion batteries
solid electrolyte interphase
thermal runaway
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
Jun 2023
Jun 2023
Historique:
revised:
20
02
2023
received:
29
12
2022
medline:
18
3
2023
pubmed:
18
3
2023
entrez:
17
3
2023
Statut:
ppublish
Résumé
Solid electrolyte interphase (SEI) plays an important role in regulating the interfacial ion transfer and safety of Lithium-ion batteries (LIBs). It is unstable and readily decomposed releasing much heat and gases and thus triggering thermal runaway. Herein, in situ heating X-ray photoelectron spectroscopy is applied to uncover the inherent thermal decomposition process of the SEI. The evolution of the composition, nanostructure, and the released gases are further probed by cryogenic transmission electron microscopy, and gas chromatography. The results show that the organic components of SEI are readily decomposed even at room temperature, releasing some flammable gases (e.g., H
Identifiants
pubmed: 36929531
doi: 10.1002/smll.202208239
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2208239Subventions
Organisme : Natural Science Foundation of Beijing
ID : Z200013
Organisme : National Key Research and Development Program of China
ID : 2022YFB2502200
Organisme : National Natural Science Foundation of China
ID : 52172257,22005334
Informations de copyright
© 2023 Wiley-VCH GmbH.
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