Recycling of Contaminated Marine Sediment and Industrial By-Products through Combined Stabilization/Solidification and Granulation Treatment.

cement-free stabilization/solidification geopolymer green remediation metal leachability waste valorization wet/cold granulation

Journal

Materials (Basel, Switzerland)
ISSN: 1996-1944
Titre abrégé: Materials (Basel)
Pays: Switzerland
ID NLM: 101555929

Informations de publication

Date de publication:
17 Mar 2023
Historique:
received: 02 01 2023
revised: 26 02 2023
accepted: 14 03 2023
medline: 30 3 2023
entrez: 29 3 2023
pubmed: 30 3 2023
Statut: epublish

Résumé

Stabilization/solidification (S/S) is becoming increasingly important, as it allows the remediation of contaminated sediments and their recovery into materials for civil engineering. This research proposes a cement-free cold granulation process for manufactured low-cost aggregates from marine sediments contaminated with organic compounds and metals. After the chemo-physical characterization of the study materials, two mix designs were prepared in a rotary plate granulator by adding two industrial by-products as geopolymer precursors, coal fly ash (CFA) and Blast Furnace Slag (BFS), but also alkaline activation solutions, water, and a fluidizer. The results indicated that sediments treated with mix 1 (i.e., with a higher percentage of water and fluidifier) represent the optimal solution in terms of metal leachability. The metal leachability was strictly influenced by aggregates' porosity, density, and microstructure. The technical performance (such as the aggregate impact value > 30%) suggested the use of granules as lightweight aggregates for pavement construction. The results indicated that cold granulation represents a sustainable solution to recycling contaminated marine sediments, CFA, and BFS into lightweight artificial aggregates.

Identifiants

pubmed: 36984279
pii: ma16062399
doi: 10.3390/ma16062399
pmc: PMC10054810
pii:
doi:

Types de publication

Journal Article

Langues

eng

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Auteurs

Francesco Todaro (F)

Department of Civil, Environmental, Land, Building Engineering and Chemistry (DICATECh), Polytechnic University of Bari, Via E. Orabona n. 4, 70125 Bari, Italy.

Francesco Colangelo (F)

Department of Engineering and INSTM Research Unit, University of Naples "Parthenope", Centro Direzionale, Isola C4, 80143 Naples, Italy.

Sabino De Gisi (S)

Department of Civil, Environmental, Land, Building Engineering and Chemistry (DICATECh), Polytechnic University of Bari, Via E. Orabona n. 4, 70125 Bari, Italy.

Ilenia Farina (I)

Department of Engineering and INSTM Research Unit, University of Naples "Parthenope", Centro Direzionale, Isola C4, 80143 Naples, Italy.

Claudio Ferone (C)

Department of Engineering and INSTM Research Unit, University of Naples "Parthenope", Centro Direzionale, Isola C4, 80143 Naples, Italy.

Claudia Labianca (C)

Department of Civil and Environmental Engineering, The Hong Kong Polytechnic University, Hung Hom, Kowloon, Hong Kong, China.

Andrea Petrella (A)

Department of Civil, Environmental, Land, Building Engineering and Chemistry (DICATECh), Polytechnic University of Bari, Via E. Orabona n. 4, 70125 Bari, Italy.

Raffaele Cioffi (R)

Department of Engineering and INSTM Research Unit, University of Naples "Parthenope", Centro Direzionale, Isola C4, 80143 Naples, Italy.

Michele Notarnicola (M)

Department of Civil, Environmental, Land, Building Engineering and Chemistry (DICATECh), Polytechnic University of Bari, Via E. Orabona n. 4, 70125 Bari, Italy.

Classifications MeSH