Peroxygenase-Catalysed Selective Oxidation of Silanes to Silanols.

Biocatalysis Oxyfunctionalization PELE Simulations Peroxygenase Silanols

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
12 Jun 2023
Historique:
received: 24 02 2023
medline: 7 4 2023
pubmed: 7 4 2023
entrez: 6 4 2023
Statut: ppublish

Résumé

A peroxygenase-catalysed hydroxylation of organosilanes is reported. The recombinant peroxygenase from Agrocybe aegerita (AaeUPO) enabled efficient conversion of a broad range of silane starting materials in attractive productivities (up to 300 mM h

Identifiants

pubmed: 37022339
doi: 10.1002/anie.202302844
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e202302844

Subventions

Organisme : European Union
ID : PeroxyZyme, No 101054658
Organisme : Guangzhou Elite Project
ID : Xiaomin Xu
Organisme : Spanish Ministery for Science and Innovation
ID : FPU19/00608
Organisme : Spanish Ministery for Science and Innovation
ID : PID2019-106370RB-I00

Informations de copyright

© 2023 The Authors. Angewandte Chemie International Edition published by Wiley-VCH GmbH.

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Auteurs

Xiaomin Xu (X)

Department of Biotechnology, Delft University of Technology, van der Maasweg 9, 2629HZ, Delft (The, Netherlands.

Jacob M A van Hengst (JMA)

Department of Biotechnology, Delft University of Technology, van der Maasweg 9, 2629HZ, Delft (The, Netherlands.

Yejia Mao (Y)

Department of Biotechnology, Delft University of Technology, van der Maasweg 9, 2629HZ, Delft (The, Netherlands.

Mireia Martinez (M)

Department of Life Sciences, Barcelona Supercomputing Center, Plaza Eusebi Güell 1-3, 08034, Barcelona, Spain.

Sergi Roda (S)

Department of Life Sciences, Barcelona Supercomputing Center, Plaza Eusebi Güell 1-3, 08034, Barcelona, Spain.

Martin Floor (M)

Department of Life Sciences, Barcelona Supercomputing Center, Plaza Eusebi Güell 1-3, 08034, Barcelona, Spain.

Victor Guallar (V)

Department of Life Sciences, Barcelona Supercomputing Center, Plaza Eusebi Güell 1-3, 08034, Barcelona, Spain.
Institució Catalana de Recerca i Estudis Avançats, Passeig de Lluís Companys, 23, 08010, Barcelona, Spain.

Caroline E Paul (CE)

Department of Biotechnology, Delft University of Technology, van der Maasweg 9, 2629HZ, Delft (The, Netherlands.

Miguel Alcalde (M)

Department of Biocatalysis, Institute of Catalysis, CSIC, Madrid, Spain.

Frank Hollmann (F)

Department of Biotechnology, Delft University of Technology, van der Maasweg 9, 2629HZ, Delft (The, Netherlands.

Classifications MeSH