Bi-Chiral Nanostructures Featuring Dynamic Optical Rotatory Dispersion for Polychromatic Light Multiplexing.

chiral nanostructures dynamic holography geometric phases light multiplexing liquid crystals

Journal

Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358

Informations de publication

Date de publication:
Aug 2023
Historique:
revised: 14 04 2023
received: 22 02 2023
medline: 9 5 2023
pubmed: 9 5 2023
entrez: 9 5 2023
Statut: ppublish

Résumé

Chiral nanostructures featuring the unique optical activity have attracted broad interests from scientists. The typical polarization rotation of transmitted light is usually wavelength dependent, namely the optical rotatory dispersion. However, its dynamic tunability and intriguing collaboration with other optical degrees of freedom, especially the highly desired spatial phase, remain elusive. Herein, a bi-chiral liquid crystalline nanostructure is proposed to induce an effect called reflective optical rotatory dispersion. Thanks to the independent manipulation of opposite-handed self-assembled helices, spin-decoupled geometric phases are induced simultaneously. These naturally unite multi-dimensions of light and versatile stimuli-responsiveness of soft matter. Dynamic holography driven by heat and electric field is demonstrated with a fast response. For polychromatic light, the hybrid multiplexed holographic painting is exhibited with fruitful tunable colors. This study extends the ingenious construction of soft chiral superstructures, presents an open-ended strategy for on-demand light control, and enlightens advanced applications of display, optical computing, and communication.

Identifiants

pubmed: 37158735
doi: 10.1002/adma.202301714
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2301714

Subventions

Organisme : National Key R&D Program of China
ID : 2021YFA1202000
Organisme : National Key R&D Program of China
ID : 2022YFA1405000
Organisme : National Natural Science Foundation of China
ID : 62222507
Organisme : National Natural Science Foundation of China
ID : 62175101
Organisme : National Natural Science Foundation of China
ID : 12004175
Organisme : Innovation Program for Quantum Science and Technology
ID : 2021ZD0301500
Organisme : Natural Science Foundation of Jiangsu Province
ID : BK20212004
Organisme : Natural Science Foundation of Jiangsu Province
ID : BK20200311

Informations de copyright

© 2023 Wiley-VCH GmbH.

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Auteurs

Si-Jia Liu (SJ)

National Laboratory of Solid State Microstructures, Key Laboratory of Intelligent Optical Sensing and Manipulation, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, 210093, China.

Lin Zhu (L)

National Laboratory of Solid State Microstructures, Key Laboratory of Intelligent Optical Sensing and Manipulation, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, 210093, China.

Yi-Heng Zhang (YH)

National Laboratory of Solid State Microstructures, Key Laboratory of Intelligent Optical Sensing and Manipulation, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, 210093, China.

Wen Chen (W)

National Laboratory of Solid State Microstructures, Key Laboratory of Intelligent Optical Sensing and Manipulation, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, 210093, China.

Dong Zhu (D)

National Laboratory of Solid State Microstructures, Key Laboratory of Intelligent Optical Sensing and Manipulation, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, 210093, China.

Peng Chen (P)

National Laboratory of Solid State Microstructures, Key Laboratory of Intelligent Optical Sensing and Manipulation, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, 210093, China.

Yan-Qing Lu (YQ)

National Laboratory of Solid State Microstructures, Key Laboratory of Intelligent Optical Sensing and Manipulation, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, 210093, China.

Classifications MeSH