Macroscopic Assembly of Chiral Hydrogen-bonded Metal-free Supramolecular Glasses for Enhanced Color-tunable Ultralong Room Temperature Phosphorescence.

Circular Polarized Luminescence Hydrogen Bonding Macroscopic Assembly Molecular Glass Ultralong Phosphorescence

Journal

Angewandte Chemie (International ed. in English)

ISSN: 1521-3773

Titre abrégé: Angew Chem Int Ed Engl

Pays: Germany

ID NLM: 0370543

Informations de publication

Date de publication:
10 Jul 2023

Historique:

received: 22 02 2023

medline: 12 5 2023

pubmed: 12 5 2023

entrez: 12 5 2023

Statut: ppublish

Résumé

Glassy materials, with desirable mechanical rigidity, shaping ability, high transparency, are attracting great interest in diverse fields. However, optically bulk molecule-based glasses are still rare, mainly due to limited monomeric species and harsh preparation conditions. Herein, we report a facile bottom-up solution fabrication process to obtain metal-free supramolecular glasses (SMGs) at the macroscopic scale using L-Histidine and hexamethylenetetramine as building blocks. The chiral SMGs possess color-tunable ultralong room temperature phosphorescence (decay lifetime up to 141.2 ms) and circular polarized luminescence (g factor up to 8.7×10

Identifiants

DOI: 10.1002/anie.202302751 PMID: 37170931

pubmed: 37170931

doi: 10.1002/anie.202302751

doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

Pagination

e202302751

Subventions

Organisme : National Natural Science Foundation of China

ID : 22275021

Organisme : Natural Science Foundation of Beijing Municipality

ID : JQ20003

Organisme : Newton Advanced Fellowship award

ID : NAF\R1\201285

Informations de copyright

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