Stability and Reversible Oxidation of Sub-Nanometric Cu

X-ray absorption spectroscopy density functional calculations nanotechnology oxidation photoelectron spectroscopy

Journal

Chemistry (Weinheim an der Bergstrasse, Germany)
ISSN: 1521-3765
Titre abrégé: Chemistry
Pays: Germany
ID NLM: 9513783

Informations de publication

Date de publication:
01 Sep 2023
Historique:
received: 14 05 2023
medline: 19 5 2023
pubmed: 19 5 2023
entrez: 19 5 2023
Statut: ppublish

Résumé

Sub-nanometer metal clusters have special physical and chemical properties, significantly different from those of nanoparticles. However, there is a major concern about their thermal stability and susceptibility to oxidation. In situ X-ray Absorption spectroscopy and Near Ambient Pressure X-ray Photoelectron spectroscopy results reveal that supported Cu

Identifiants

pubmed: 37204268
doi: 10.1002/chem.202301517
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e202301517

Subventions

Organisme : Agencia Nacional de Promoción Científica y Tecnológica
ID : PICT 2017-1220
Organisme : Agencia Nacional de Promoción Científica y Tecnológica
ID : PICT 2017-3944
Organisme : Agencia Nacional de Promoción Científica y Tecnológica
ID : PICT 2019-0784
Organisme : Agencia Estatal de Investigación
ID : PID2019-107115GB-C21
Organisme : Agencia Estatal de Investigación
ID : PID2020-117605GB-I00
Organisme : Austrian Science Fund
ID : P29893-N36
Organisme : European Cooperation in Science and Technology
ID : CM1405 "Molecules in Motion" (MOLIM)
Organisme : European Cooperation in Science and Technology
ID : COST Action CA21101 "Confined molecular systems: from a new generation of materialsto the stars"
Organisme : Xunta de Galicia
ID : Grupos Ref. Comp. 2021 - ED431C 2021/16
Organisme : Universidad Nacional de La Plata
ID : 11/X937
Organisme : Ministerio de Ciencia, Innovación y Universidades
ID : TED2021-131899B-I00/MCIN/AEI/10.13039/501100011033/ Unión Europea NextGenerationEU/PRTR
Organisme : HORIZON EUROPE Framework Programme
ID : EU Doctoral Network PHYMOL 101073474 (project call reference HORIZON-MSCA-2021-DN-01

Informations de copyright

© 2023 The Authors. Chemistry - A European Journal published by Wiley-VCH GmbH.

Références

J Phys Condens Matter. 2019 Apr 10;31(14):144002
pubmed: 30625421
J Phys Chem A. 2021 Apr 15;125(14):2836-2848
pubmed: 33787276
J Chem Phys. 2015 Sep 14;143(10):102804
pubmed: 26373997
J Chem Phys. 2015 Nov 21;143(19):194701
pubmed: 26590547
J Am Chem Soc. 2015 Mar 25;137(11):3894-900
pubmed: 25747902
Nat Commun. 2016 Oct 24;7:13240
pubmed: 27775036
J Chem Phys. 2010 Apr 21;132(15):154104
pubmed: 20423165
J Comput Chem. 2011 May;32(7):1456-65
pubmed: 21370243
J Chem Phys. 2007 Apr 14;126(14):144111
pubmed: 17444705
J Chem Phys. 2018 Mar 21;148(11):110901
pubmed: 29566496
J Synchrotron Radiat. 2005 Jul;12(Pt 4):537-41
pubmed: 15968136
Chem Rev. 2018 May 23;118(10):4981-5079
pubmed: 29658707
Anal Bioanal Chem. 2004 Aug;379(7-8):920-30
pubmed: 15338088
Chemistry. 2023 Sep 1;29(49):e202301517
pubmed: 37204268
J Chem Phys. 2019 Apr 21;150(15):154122
pubmed: 31005066
Chem Rev. 2018 Jun 13;118(11):5755-5870
pubmed: 29812916
J Am Chem Soc. 2020 Feb 12;142(6):2857-2867
pubmed: 31955572
ACS Omega. 2021 Jun 07;6(24):16165-16175
pubmed: 34179662
J Am Chem Soc. 2015 Sep 2;137(34):11186-90
pubmed: 26275662
Phys Rev Lett. 2013 Sep 27;111(13):135501
pubmed: 24116790
J Phys Chem Lett. 2018 Jun 7;9(11):3035-3042
pubmed: 29665684
J Chem Phys. 2020 Apr 14;152(14):144107
pubmed: 32295355
Phys Chem Chem Phys. 2013 Dec 21;15(47):20727-34
pubmed: 24196250
Phys Chem Chem Phys. 2014 Dec 28;16(48):26500-5
pubmed: 25030778
Phys Rev B Condens Matter. 1989 Jan 15;39(3):1541-1545
pubmed: 9948365
Phys Chem Chem Phys. 2005 Sep 21;7(18):3297-305
pubmed: 16240044
Nat Nanotechnol. 2015 Jul;10(7):577-88
pubmed: 26139144
J Phys Chem Lett. 2020 Apr 16;11(8):3089-3094
pubmed: 32227852
Phys Chem Chem Phys. 2018 Jul 18;20(28):19110-19119
pubmed: 29974080
J Mater Chem A Mater. 2019 Apr 7;7(13):7489-7500
pubmed: 31007927
Phys Rev Lett. 1996 Oct 28;77(18):3865-3868
pubmed: 10062328
Acc Chem Res. 2020 Feb 18;53(2):447-458
pubmed: 31977181
Phys Chem Chem Phys. 2018 Dec 12;20(48):30437-30444
pubmed: 30500006
J Phys Chem C Nanomater Interfaces. 2019 Sep 19;123(37):23064-23074
pubmed: 31598186
J Phys Chem C Nanomater Interfaces. 2019 Nov 7;123(44):27064-27072
pubmed: 33101568
J Am Chem Soc. 2013 Nov 20;135(46):17417-31
pubmed: 24102191
J Phys Chem B. 2006 Aug 24;110(33):16591-9
pubmed: 16913794

Auteurs

David Buceta (D)

Department of Physical Chemistry, Nanomag Laboratory, Universidad de Santiago de Compostela, 15782, Santiago de Compostela, Spain.

Shahana Huseyinova (S)

Department of Physical Chemistry, Nanomag Laboratory, Universidad de Santiago de Compostela, 15782, Santiago de Compostela, Spain.

Miguel Cuerva (M)

Department of Physical Chemistry, Nanomag Laboratory, Universidad de Santiago de Compostela, 15782, Santiago de Compostela, Spain.

Héctor Lozano (H)

Department of Physical Chemistry, Nanomag Laboratory, Universidad de Santiago de Compostela, 15782, Santiago de Compostela, Spain.

Lisandro J Giovanetti (LJ)

Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas (INIFTA), Dto. de Química, Facultad de Ciencias Exactas, UNLP and CONICET, Diag. 113 y 64., 1900, La Plata, Argentina.

José M Ramallo-López (JM)

Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas (INIFTA), Dto. de Química, Facultad de Ciencias Exactas, UNLP and CONICET, Diag. 113 y 64., 1900, La Plata, Argentina.

Patricia López-Caballero (P)

Instituto de Física Fundamental (AbinitSim Unit), CSIC, Serrano 123, 28006, Madrid, Spain.

Alexandre Zanchet (A)

Instituto de Física Fundamental (AbinitSim Unit), CSIC, Serrano 123, 28006, Madrid, Spain.

Alexander O Mitrushchenkov (AO)

MSME, Univ Gustave Eiffel, UPEC, CNRS, 77454, Marne-la-Vallée, France.

Andreas W Hauser (AW)

Institute of Experimental Physics, Graz University of Technology, Petersgasse 16, 8010, Graz, Austria.

Giampaolo Barone (G)

Department of Biological, Chemical and Pharmaceutical Sciences and Technologies, University of Palermo, 90128, Palermo, Italy.

Cristián Huck-Iriart (C)

Laboratorio de Cristalografía Aplicada, Escuela de Ciencia y Tecnología, Universidad Nacional de San Martín (UNSAM), Campus Miguelete, 25 de Mayo y Francia, 1650, San Martín, Provincia, Buenos Aires, Argentina.
ALBA Synchrotron Light Source, Carrer de la Llum 2-26, 08290, Cerdanyola del Vallès, Barcelona, Spain.

Carlos Escudero (C)

ALBA Synchrotron Light Source, Carrer de la Llum 2-26, 08290, Cerdanyola del Vallès, Barcelona, Spain.

Juan Carlos Hernández-Garrido (JC)

Department of Material Science and Metallurgic Engineering and Inorganic Chemistry, Faculty of Science, University of Cádiz, 11510, Puerto Real, Cádiz, Spain.

José Juan Calvino (JJ)

Department of Material Science and Metallurgic Engineering and Inorganic Chemistry, Faculty of Science, University of Cádiz, 11510, Puerto Real, Cádiz, Spain.

Miguel López-Haro (M)

Department of Material Science and Metallurgic Engineering and Inorganic Chemistry, Faculty of Science, University of Cádiz, 11510, Puerto Real, Cádiz, Spain.

María Pilar de Lara-Castells (MP)

Instituto de Física Fundamental (AbinitSim Unit), CSIC, Serrano 123, 28006, Madrid, Spain.

Félix G Requejo (FG)

Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas (INIFTA), Dto. de Química, Facultad de Ciencias Exactas, UNLP and CONICET, Diag. 113 y 64., 1900, La Plata, Argentina.

M Arturo López-Quintela (MA)

Department of Physical Chemistry, Nanomag Laboratory, Universidad de Santiago de Compostela, 15782, Santiago de Compostela, Spain.

Classifications MeSH