Coherent control of an ultrabright single spin in hexagonal boron nitride at room temperature.

Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
20 May 2023
Historique:
received: 13 09 2022
accepted: 10 05 2023
medline: 21 5 2023
pubmed: 21 5 2023
entrez: 20 5 2023
Statut: epublish

Résumé

Hexagonal boron nitride (hBN) is a remarkable two-dimensional (2D) material that hosts solid-state spins and has great potential to be used in quantum information applications, including quantum networks. However, in this application, both the optical and spin properties are crucial for single spins but have not yet been discovered simultaneously for hBN spins. Here, we realize an efficient method for arraying and isolating the single defects of hBN and use this method to discover a new spin defect with a high probability of 85%. This single defect exhibits outstanding optical properties and an optically controllable spin, as indicated by the observed significant Rabi oscillation and Hahn echo experiments at room temperature. First principles calculations indicate that complexes of carbon and oxygen dopants may be the origin of the single spin defects. This provides a possibility for further addressing spins that can be optically controlled.

Identifiants

DOI: 10.1038/s41467-023-38672-6 PMID: 37210408 PMC: PMC10199889
pubmed: 37210408
doi: 10.1038/s41467-023-38672-6
pii: 10.1038/s41467-023-38672-6
pmc: PMC10199889
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

2893

Subventions

Organisme : National Natural Science Foundation of China (National Science Foundation of China)
ID : 11821404

Informations de copyright

© 2023. The Author(s).

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Auteurs

Nai-Jie Guo (NJ)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.

Song Li (S)

Wigner Research Centre for Physics, Post Office Box 49, H-1525Budapest, Hungary.

Wei Liu (W)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.

Yuan-Ze Yang (YZ)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.

Xiao-Dong Zeng (XD)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.

Shang Yu (S)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.

Yu Meng (Y)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.

Zhi-Peng Li (ZP)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.

Zhao-An Wang (ZA)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.

Lin-Ke Xie (LK)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.

Rong-Chun Ge (RC)

College of Physics, Sichuan University, Chengdu, 610064, China.

Jun-Feng Wang (JF)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.
College of Physics, Sichuan University, Chengdu, 610064, China.

Qiang Li (Q)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.

Jin-Shi Xu (JS)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.
ORCID: 0000-0003-0528-1000

Yi-Tao Wang (YT)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China. yitao@ustc.edu.cn.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China. yitao@ustc.edu.cn.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China. yitao@ustc.edu.cn.
ORCID: 0000-0003-3028-0923

Jian-Shun Tang (JS)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China. tjs@ustc.edu.cn.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China. tjs@ustc.edu.cn.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China. tjs@ustc.edu.cn.
ORCID: 0000-0002-2191-8350

Adam Gali (A)

Wigner Research Centre for Physics, Post Office Box 49, H-1525Budapest, Hungary. gali.adam@wigner.hu.
Department of Atomic Physics, Institute of Physics, Budapest University of Technology and Economics, Muegyetem rakpart 3, H-1111Budapest, Hungary. gali.adam@wigner.hu.
ORCID: 0000-0002-3339-5470

Chuan-Feng Li (CF)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China. cfli@ustc.edu.cn.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China. cfli@ustc.edu.cn.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China. cfli@ustc.edu.cn.
ORCID: 0000-0001-6815-8929

Guang-Can Guo (GC)

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui, 230026, China.
CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui, 230026, China.
Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088, China.

Classifications MeSH