Ultrafast electron diffraction instrument for gas and condensed matter samples.


Journal

The Review of scientific instruments
ISSN: 1089-7623
Titre abrégé: Rev Sci Instrum
Pays: United States
ID NLM: 0405571

Informations de publication

Date de publication:
01 May 2023
Historique:
received: 15 02 2023
accepted: 04 05 2023
medline: 23 5 2023
pubmed: 23 5 2023
entrez: 23 5 2023
Statut: ppublish

Résumé

We report the modification of a gas phase ultrafast electron diffraction (UED) instrument that enables experiments with both gas and condensed matter targets, where a time-resolved experiment with sub-picosecond resolution is demonstrated with solid state samples. The instrument relies on a hybrid DC-RF acceleration structure to deliver femtosecond electron pulses on the target, which is synchronized with femtosecond laser pulses. The laser pulses and electron pulses are used to excite the sample and to probe the structural dynamics, respectively. The new system is added with capabilities to perform transmission UED on thin solid samples. It allows for cooling samples to cryogenic temperatures and to carry out time-resolved measurements. We tested the cooling capability by recording diffraction patterns of temperature dependent charge density waves in 1T-TaS2. The time-resolved capability is experimentally verified by capturing the dynamics in photoexcited single-crystal gold.

Identifiants

pubmed: 37219385
pii: 2892277
doi: 10.1063/5.0146577
pii:
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Informations de copyright

© 2023 Author(s). Published under an exclusive license by AIP Publishing.

Auteurs

Yibo Wang (Y)

Department of Physics and Astronomy, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.

Sajib Kumar Saha (SK)

Department of Physics and Astronomy, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.

Tianlin Li (T)

Department of Physics and Astronomy, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.

Yanwei Xiong (Y)

Department of Physics and Astronomy, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.

Kyle Wilkin (K)

Department of Physics and Astronomy, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.

Anil Adhikari (A)

Department of Physics and Astronomy, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.

Michael Loes (M)

Department of Chemistry, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.

Jehad Abourahma (J)

Department of Chemistry, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.

Xia Hong (X)

Department of Physics and Astronomy, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.
Nebraska Center for Materials and Nanoscience, University of Nebraska-Lincoln, Lincoln, Nebraska 65588-0298, USA.

Shireen Adenwalla (S)

Department of Physics and Astronomy, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.

Alexander Sinitskii (A)

Department of Chemistry, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.

Martin Centurion (M)

Department of Physics and Astronomy, University of Nebraska-Lincoln, 855 N 16th Street, Lincoln, Nebraska 68588-0298, USA.

Classifications MeSH