Rotational and dilational reconstruction in transition metal dichalcogenide moiré bilayers.


Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
24 May 2023
Historique:
received: 15 12 2022
accepted: 03 05 2023
medline: 25 5 2023
pubmed: 25 5 2023
entrez: 24 5 2023
Statut: epublish

Résumé

Lattice reconstruction and corresponding strain accumulation plays a key role in defining the electronic structure of two-dimensional moiré superlattices, including those of transition metal dichalcogenides (TMDs). Imaging of TMD moirés has so far provided a qualitative understanding of this relaxation process in terms of interlayer stacking energy, while models of the underlying deformation mechanisms have relied on simulations. Here, we use interferometric four-dimensional scanning transmission electron microscopy to quantitatively map the mechanical deformations through which reconstruction occurs in small-angle twisted bilayer MoS

Identifiants

pubmed: 37225701
doi: 10.1038/s41467-023-38504-7
pii: 10.1038/s41467-023-38504-7
pmc: PMC10209090
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

2989

Subventions

Organisme : National Science Foundation (NSF)
ID : DMR-2238196
Organisme : National Science Foundation (NSF)
ID : OIA-1921199
Organisme : Gordon and Betty Moore Foundation (Gordon E. and Betty I. Moore Foundation)
ID : 10637
Organisme : Canadian Institute for Advanced Research (L'Institut Canadien de Recherches Avancées)
ID : GS21-011
Organisme : W. M. Keck Foundation (W.M. Keck Foundation)
ID : 993922
Organisme : U.S. Department of Defense (United States Department of Defense)
ID : FA9550-21-F-0003
Organisme : Ministry of Education, Culture, Sports, Science and Technology (MEXT)
ID : JPMXP0112101001
Organisme : MEXT | Japan Society for the Promotion of Science (JSPS)
ID : 20H00354
Organisme : MEXT | Japan Society for the Promotion of Science (JSPS)
ID : 21H05233
Organisme : U.S. Department of Energy (DOE)
ID : DE-AC02-05CH11231

Informations de copyright

© 2023. The Author(s).

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Auteurs

Madeline Van Winkle (M)

Department of Chemistry, University of California, Berkeley, CA, 94720, USA.

Isaac M Craig (IM)

Department of Chemistry, University of California, Berkeley, CA, 94720, USA.
Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.
Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

Stephen Carr (S)

Department of Physics, Brown University, Providence, RI, 02912, USA.
Brown Theoretical Physics Center, Brown University, Providence, RI, 02912, USA.

Medha Dandu (M)

Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

Karen C Bustillo (KC)

Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

Jim Ciston (J)

Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

Colin Ophus (C)

Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

Takashi Taniguchi (T)

International Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan.

Kenji Watanabe (K)

Research for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan.

Archana Raja (A)

Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

Sinéad M Griffin (SM)

Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.
Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.

D Kwabena Bediako (DK)

Department of Chemistry, University of California, Berkeley, CA, 94720, USA. bediako@berkeley.edu.
Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA. bediako@berkeley.edu.

Classifications MeSH