Local Photochemical Nanoscopy of Hot-Carrier-Driven Catalytic Reactions Using Plasmonic Nanosystems.

hot charge carriers in situ nanoscopy photocatalysis plasmonics scanning electrochemical microscopy

Journal

ACS nano
ISSN: 1936-086X
Titre abrégé: ACS Nano
Pays: United States
ID NLM: 101313589

Informations de publication

Date de publication:
27 Jun 2023
Historique:
medline: 13 6 2023
pubmed: 13 6 2023
entrez: 13 6 2023
Statut: ppublish

Résumé

Nanoscale investigation of the reactivity of photocatalytic systems is crucial for their fundamental understanding and improving their design and applicability. Here, we present a photochemical nanoscopy technique that unlocks the local spatial detection of molecular products during plasmonic hot-carrier-driven photocatalytic reactions with nanometric precision. By applying the methodology to Au/TiO

Identifiants

pubmed: 37310716
doi: 10.1021/acsnano.3c01009
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

11427-11438

Auteurs

Olivier Henrotte (O)

Czech Advanced Technology and Research Institute, Regional Centre of Advanced Technologies and Materials Department, Palacký University Olomouc, Šlechtitelů 27, Olomouc 78371, Czech Republic.

Eva Yazmin Santiago (EY)

Department of Physics and Astronomy, Nanoscale and Quantum Phenomena Institute, Ohio University, Athens, Ohio 45701, United States.

Artur Movsesyan (A)

Department of Physics and Astronomy, Nanoscale and Quantum Phenomena Institute, Ohio University, Athens, Ohio 45701, United States.
Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China.

Luca Mascaretti (L)

Czech Advanced Technology and Research Institute, Regional Centre of Advanced Technologies and Materials Department, Palacký University Olomouc, Šlechtitelů 27, Olomouc 78371, Czech Republic.

Morteza Afshar (M)

Czech Advanced Technology and Research Institute, Regional Centre of Advanced Technologies and Materials Department, Palacký University Olomouc, Šlechtitelů 27, Olomouc 78371, Czech Republic.

Alessandro Minguzzi (A)

Laboratory of Applied Electrochemistry, Dipartimento di Chimica, Università degli Studi di Milano, via Golgi 19, Milano 20133, Italy.
Consorzio Interuniversitario Nazionale per la Scienza e Tecnologia dei Materiali, via Giusti 9, Firenze 50121, Italy.

Alberto Vertova (A)

Laboratory of Applied Electrochemistry, Dipartimento di Chimica, Università degli Studi di Milano, via Golgi 19, Milano 20133, Italy.
Consorzio Interuniversitario Nazionale per la Scienza e Tecnologia dei Materiali, via Giusti 9, Firenze 50121, Italy.

Zhiming M Wang (ZM)

Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China.

Radek Zbořil (R)

Czech Advanced Technology and Research Institute, Regional Centre of Advanced Technologies and Materials Department, Palacký University Olomouc, Šlechtitelů 27, Olomouc 78371, Czech Republic.
CEET, Nanotechnology Centre, VŠB-Technical University of Ostrava, 17. Listopadu 2172/15, Ostrava-Poruba 708 00, Czech Republic.

Štěpán Kment (Š)

Czech Advanced Technology and Research Institute, Regional Centre of Advanced Technologies and Materials Department, Palacký University Olomouc, Šlechtitelů 27, Olomouc 78371, Czech Republic.
CEET, Nanotechnology Centre, VŠB-Technical University of Ostrava, 17. Listopadu 2172/15, Ostrava-Poruba 708 00, Czech Republic.

Alexander O Govorov (AO)

Department of Physics and Astronomy, Nanoscale and Quantum Phenomena Institute, Ohio University, Athens, Ohio 45701, United States.

Alberto Naldoni (A)

Czech Advanced Technology and Research Institute, Regional Centre of Advanced Technologies and Materials Department, Palacký University Olomouc, Šlechtitelů 27, Olomouc 78371, Czech Republic.
Department of Chemistry and NIS Centre, University of Turin, Turin 10125, Italy.

Classifications MeSH