Bottom-Up Preparation of Phase-Separated Polymersomes.

drug delivery phase separation polymersomes self-assembly vesicles

Journal

Macromolecular bioscience
ISSN: 1616-5195
Titre abrégé: Macromol Biosci
Pays: Germany
ID NLM: 101135941

Informations de publication

Date de publication:
08 2023
Historique:
revised: 20 05 2023
received: 20 02 2023
medline: 21 8 2023
pubmed: 14 6 2023
entrez: 14 6 2023
Statut: ppublish

Résumé

A bottom-up approach to fabricating monodisperse, two-component polymersomes that possess phase-separated ("patchy") chemical topology is presented. This approach is compared with already-existing top-down preparation methods for patchy polymer vesicles, such as film rehydration. These findings demonstrate a bottom-up, solvent-switch self-assembly approach that produces a high yield of nanoparticles of the target size, morphology, and surface topology for drug delivery applications, in this case patchy polymersomes of a diameter of ≈50 nm. In addition, an image processing algorithm to automatically calculate polymersome size distributions from transmission electron microscope images based on a series of pre-processing steps, image segmentation, and round object identification is presented.

Identifiants

pubmed: 37315231
doi: 10.1002/mabi.202300068
doi:

Substances chimiques

Polymers 0
Solvents 0

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2300068

Informations de copyright

© 2023 Wiley-VCH GmbH.

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Auteurs

Safa Almadhi (S)

Department of Chemistry, University College London, London, WC1H 0AJ, UK.

Joe Forth (J)

Department of Chemistry, University College London, London, WC1H 0AJ, UK.

Laura Rodriguez-Arco (L)

Department of Chemistry, University College London, London, WC1H 0AJ, UK.
Department of Applied Physics, Faculty of Sciences, University of Granada, Granada, 18071, Spain.

Aroa Duro-Castano (A)

Department of Chemistry, University College London, London, WC1H 0AJ, UK.
Curapath, Valencia, 46980, Spain.

Ian Williams (I)

Department of Chemistry, University College London, London, WC1H 0AJ, UK.
Department of Physics, University of Surrey, Guildford, GU2 7XH, UK.
Institute for Bioengineering of Catalonia, The Barcelona Institute of Science and Technology, Barcelona, 08028, Spain.

Lorena Ruiz-Pérez (L)

Department of Chemistry, University College London, London, WC1H 0AJ, UK.
Institute for Bioengineering of Catalonia, The Barcelona Institute of Science and Technology, Barcelona, 08028, Spain.

Giuseppe Battaglia (G)

Department of Chemistry, University College London, London, WC1H 0AJ, UK.
Institute for Bioengineering of Catalonia, The Barcelona Institute of Science and Technology, Barcelona, 08028, Spain.
Catalan Institution of Research and Advanced Studies, Barcelona, 08010, Spain.

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