Half-Electrolysis of Water with the Aid of a Supercapacitor Electrode.


Journal

ACS applied energy materials
ISSN: 2574-0962
Titre abrégé: ACS Appl Energy Mater
Pays: United States
ID NLM: 101718976

Informations de publication

Date de publication:
12 Jun 2023
Historique:
received: 07 03 2023
accepted: 04 05 2023
medline: 16 6 2023
pubmed: 16 6 2023
entrez: 16 6 2023
Statut: epublish

Résumé

Half-electrolysis runs one desirable half-cell reaction with the aid of a counter supercapacitor electrode which replaces the other unwanted half-cell reaction occurred inevitably in conventional electrolysis. Herein, it is developed to complete the whole cell reaction of water electrolysis, in alternative steps, with a capacitive activated carbon (AC) electrode and an electrolysis Pt electrode. When positively charging the AC electrode, a hydrogen evolution reaction occurs at the Pt electrode. By reversing the current, the charge stored in the AC electrode is discharged to assist the oxygen evolution reaction on the same Pt electrode. Consecutive completion of the two processes realizes the overall reaction of water electrolysis. This strategy leads to stepwise production of H

Identifiants

pubmed: 37323209
doi: 10.1021/acsaem.3c00615
pmc: PMC10265655
doi:

Types de publication

Journal Article

Langues

eng

Pagination

6104-6110

Informations de copyright

© 2023 The Authors. Published by American Chemical Society.

Déclaration de conflit d'intérêts

The authors declare the following competing financial interest(s): The authors declare the competing financial interests with CN patents (201910155530.6) and (201910155553.7).

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Auteurs

Yao Chen (Y)

The State Key Laboratory of Refractories and Metallurgy, College of Materials and Metallurgy, Wuhan University of Science and Technology, Wuhan 430081, P. R. China.

George Zheng Chen (GZ)

Department of Chemical and Environmental Engineering, Faculty of Engineering, University of Nottingham, Nottingham NG2 7RD, U.K.

Classifications MeSH