Multisite PCET with photocharged carbon nitride in dark.
PCET
carbon nitride
photocatalysis
photocharging
poly(heptazine imide)
thermochemistry
Journal
Exploration (Beijing, China)
ISSN: 2766-2098
Titre abrégé: Exploration (Beijing)
Pays: China
ID NLM: 9918383883006676
Informations de publication
Date de publication:
Dec 2021
Dec 2021
Historique:
received:
30
07
2021
accepted:
15
11
2021
medline:
16
12
2021
pubmed:
16
12
2021
entrez:
16
6
2023
Statut:
epublish
Résumé
A combination of photochemistry and proton coupled electron transfer (PCET) is a primary strategy employed by biochemical systems and synthetic chemistry to enable uphill reactions under mild conditions. Degenerate nanometer-sized n-type semiconductor nanoparticles (SCNPs) with the Fermi level above the bottom of the conduction band are strongly reducing and act more like metals than semiconductors. Application of the degenerate SCNPs is limited to few examples. Herein, we load microporous potassium poly(heptazine imide) (K-PHI) nanoparticles with electrons (e
Identifiants
pubmed: 37323696
doi: 10.1002/EXP.20210063
pii: EXP236
pmc: PMC10190955
doi:
Types de publication
Journal Article
Langues
eng
Pagination
20210063Informations de copyright
© 2021 The Authors. Exploration published by Henan University and John Wiley & Sons Australia, Ltd.
Déclaration de conflit d'intérêts
A patent WO/2019/081036 has been filed by Max Planck Gesellschaft zur Förderung der Wissenschaften E.V. in which Aleksandr Savateev and Markus Antonietti are listed as co‐authors.
Références
Org Biomol Chem. 2016 Sep 26;14(38):9151-9157
pubmed: 27714249
Chemistry. 2015 Oct 12;21(42):14764-7
pubmed: 26332922
Environ Sci Technol. 2013 Dec 17;47(24):14194-203
pubmed: 24237268
Nat Commun. 2020 Mar 13;11(1):1387
pubmed: 32170119
J Phys Chem Lett. 2012 Mar 1;3(5):663-72
pubmed: 26286163
Inorg Chem. 1999 Jun 14;38(12):2760-2761
pubmed: 11671018
Angew Chem Int Ed Engl. 2021 Mar 22;60(13):7436-7443
pubmed: 33259655
Acc Chem Res. 2003 Apr;36(4):255-63
pubmed: 12693923
J Am Chem Soc. 2020 Feb 5;142(5):2093-2099
pubmed: 31951393
Chem Sci. 2018 Mar 14;9(14):3584-3591
pubmed: 29780491
European J Org Chem. 2017 Apr 18;2017(15):2056-2071
pubmed: 30147436
J Am Chem Soc. 2016 Jul 27;138(29):9183-92
pubmed: 27337491
Chempluschem. 2020 Nov;85(11):2499-2517
pubmed: 33215877
Chem Mater. 2019 Sep 24;31(18):7478-7486
pubmed: 31582875
Angew Chem Int Ed Engl. 2020 Aug 24;59(35):15061-15068
pubmed: 32412175
Angew Chem Int Ed Engl. 2017 Jan 9;56(2):510-514
pubmed: 27930846
J Am Chem Soc. 2005 Mar 23;127(11):3928-34
pubmed: 15771529
Angew Chem Int Ed Engl. 2015 Jul 20;54(30):8828-32
pubmed: 26082970
J Am Chem Soc. 2015 Sep 2;137(34):11163-9
pubmed: 26263400
J Am Chem Soc. 2018 Jul 18;140(28):8924-8933
pubmed: 29920088
Nat Commun. 2019 Feb 26;10(1):945
pubmed: 30808862
Chem Rev. 2010 Dec 8;110(12):6961-7001
pubmed: 20925411
Science. 2012 Jun 8;336(6086):1298-301
pubmed: 22679095
Phys Rev Lett. 2007 May 4;98(18):186804
pubmed: 17501594
Angew Chem Int Ed Engl. 2018 Dec 3;57(49):15936-15947
pubmed: 30066478
Chem Commun (Camb). 2018 Mar 27;54(26):3215-3218
pubmed: 29393332
Inorg Chem. 2013 May 20;52(10):5924-30
pubmed: 23651218
Chem Soc Rev. 2021 Mar 1;50(4):2244-2259
pubmed: 33313618
Phys Chem Chem Phys. 2017 Nov 8;19(43):29053-29056
pubmed: 29083014
Science. 2014 Nov 7;346(6210):725-8
pubmed: 25378618
Angew Chem Int Ed Engl. 2013 Nov 25;52(48):12636-40
pubmed: 24123574
Nat Chem. 2012 Oct;4(10):854-9
pubmed: 23001000
Top Curr Chem (Cham). 2016 Jun;374(3):30
pubmed: 27573270
Phys Chem Chem Phys. 2013 Jul 7;15(25):10335-8
pubmed: 23715241
Annu Rev Biochem. 2009;78:673-99
pubmed: 19344235
Adv Mater. 2020 Mar;32(10):e1908140
pubmed: 31995254
J Phys Chem Lett. 2020 Sep 17;11(18):7687-7691
pubmed: 32838515
Nat Mater. 2011 May;10(5):361-6
pubmed: 21478881
Nat Commun. 2018 Jan 4;9(1):60
pubmed: 29302040
Acc Chem Res. 2016 Aug 16;49(8):1546-56
pubmed: 27472068
J Am Chem Soc. 2013 Nov 6;135(44):16569-77
pubmed: 24050304