Synthesis of hyocholic acid and its derivatization with sodium periodate to distinguish it from cholic acid by mass spectrometry.

Bile acids Hyocholic Acid Mass Spectrometry Ox Bile Oxidation Synthesis

Journal

Steroids
ISSN: 1878-5867
Titre abrégé: Steroids
Pays: United States
ID NLM: 0404536

Informations de publication

Date de publication:
09 2023
Historique:
received: 07 04 2023
revised: 15 06 2023
accepted: 16 06 2023
medline: 27 7 2023
pubmed: 20 6 2023
entrez: 19 6 2023
Statut: ppublish

Résumé

Low concentrations of hyocholic acid in human serum has been linked to diabetes. Due to its important role in human health, we were interested in synthesizing hyocholic acid to explore potential biochemical properties of this bile acid. Here, a synthesis of hyocholic acid is reported from chenodeoxycholic acid. The key step was a Rubottom oxidation of a silyl enol ether intermediate to directly incorporate the oxygen at C6. Furthermore, the synthesized hyocholic acid product was treated with NaIO

Identifiants

pubmed: 37336340
pii: S0039-128X(23)00088-0
doi: 10.1016/j.steroids.2023.109260
pii:
doi:

Substances chimiques

Cholic Acid G1JO7801AE
muricholic acid 39016-49-4
metaperiodate B45A1BUM4Q
Cholic Acids 0
Bile Acids and Salts 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

109260

Informations de copyright

Copyright © 2023 Elsevier Inc. All rights reserved.

Déclaration de conflit d'intérêts

Declaration of Competing Interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

Auteurs

Tu M Ho (TM)

Department of Chemistry, The University of Texas at San Antonio (UTSA), San Antonio, TX 78249, United States.

Hadi D Arman (HD)

Department of Chemistry, The University of Texas at San Antonio (UTSA), San Antonio, TX 78249, United States.

Francis K Yoshimoto (FK)

Department of Chemistry, The University of Texas at San Antonio (UTSA), San Antonio, TX 78249, United States. Electronic address: francis.yoshimoto@utsa.edu.

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Classifications MeSH