Quantum Sensing of Electric Fields Using Spin-Correlated Radical Ion Pairs.


Journal

Journal of the American Chemical Society
ISSN: 1520-5126
Titre abrégé: J Am Chem Soc
Pays: United States
ID NLM: 7503056

Informations de publication

Date de publication:
12 Jul 2023
Historique:
medline: 26 6 2023
pubmed: 26 6 2023
entrez: 26 6 2023
Statut: ppublish

Résumé

Quantum sensing affords the possibility of using quantum entanglement to probe electromagnetic fields with exquisite sensitivity. In this work, we show that a photogenerated spin-correlated radical ion pair (SCRP) can be used to sense an electric field change created at one radical ion of the pair using molecular recognition. The SCRP is generated within a covalent donor-chromophore-acceptor system PXX-PMI-NDI,

Identifiants

pubmed: 37364237
doi: 10.1021/jacs.3c04212
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

14922-14931

Auteurs

Fangbai Xie (F)

Department of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.
Center for Molecular Quantum Transduction and Institute for Sustainability and Energy at Northwestern, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.

Haochuan Mao (H)

Department of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.
Center for Molecular Quantum Transduction and Institute for Sustainability and Energy at Northwestern, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.

Chenjian Lin (C)

Department of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.
Center for Molecular Quantum Transduction and Institute for Sustainability and Energy at Northwestern, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.

Yuanning Feng (Y)

Department of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.

J Fraser Stoddart (JF)

Department of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.
School of Chemistry, University of New South Wales, Sydney, New South Wales 2052, Australia.
Stoddart Institute of Molecular Science, Department of Chemistry, Zhejiang University, Hangzhou 310027, China.
ZJU-Hangzhou Global Scientific and Technological Innovation Center, Hangzhou 311215, China.

Ryan M Young (RM)

Department of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.
Center for Molecular Quantum Transduction and Institute for Sustainability and Energy at Northwestern, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.

Michael R Wasielewski (MR)

Department of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.
Center for Molecular Quantum Transduction and Institute for Sustainability and Energy at Northwestern, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208-3113, United States.

Classifications MeSH