Impact of bimetallic interface design on heat generation in plasmonic Au/Pd nanostructures studied by single-particle thermometry.
Journal
Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555
Informations de publication
Date de publication:
27 Jun 2023
27 Jun 2023
Historique:
received:
03
11
2022
accepted:
17
05
2023
medline:
28
6
2023
pubmed:
28
6
2023
entrez:
27
6
2023
Statut:
epublish
Résumé
Localized surface plasmons are lossy and generate heat. However, accurate measurement of the temperature of metallic nanoparticles under illumination remains an open challenge, creating difficulties in the interpretation of results across plasmonic applications. Particularly, there is a quest for understanding the role of temperature in plasmon-assisted catalysis. Bimetallic nanoparticles combining plasmonic with catalytic metals are raising increasing interest in artificial photosynthesis and the production of solar fuels. Here, we perform single-particle thermometry measurements to investigate the link between morphology and light-to-heat conversion of colloidal Au/Pd nanoparticles with two different configurations: core-shell and core-satellite. It is observed that the inclusion of Pd as a shell strongly reduces the photothermal response in comparison to the bare cores, while the inclusion of Pd as satellites keeps photothermal properties almost unaffected. These results contribute to a better understanding of energy conversion processes in plasmon-assisted catalysis.
Identifiants
pubmed: 37369657
doi: 10.1038/s41467-023-38982-9
pii: 10.1038/s41467-023-38982-9
pmc: PMC10300195
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
3813Subventions
Organisme : Deutscher Akademischer Austauschdienst (German Academic Exchange Service)
ID : PRIME fellowship Julian Gargiulo
Organisme : Alexander von Humboldt-Stiftung (Alexander von Humboldt Foundation)
ID : Julian Gargiulo
Organisme : Royal Society of Chemistry (RSC)
ID : Research Fund R20-7244
Organisme : Ministry of Science, Technology and Productive Innovation, Argentina | Agencia Nacional de Promoción Científica y Tecnológica (National Agency for Science and Technology, Argentina)
ID : PICT-2020-SERIEA-02966
Organisme : Consellería de Cultura, Educación e Ordenación Universitaria, Xunta de Galicia (Ministry of Culture, Education and University Planning, Government of Galicia)
ID : Postdoctoral fellowship Ana Sousa-Castillo
Organisme : Deutsche Forschungsgemeinschaft (German Research Foundation)
ID : Germany's Excellence Strategy, EXC 2089/1-390776260
Informations de copyright
© 2023. The Author(s).
Références
ACS Nano. 2022 Aug 23;16(8):12377-12389
pubmed: 35894585
J Chem Phys. 2021 Aug 14;155(6):060901
pubmed: 34391373
Chem Rev. 2019 Jul 10;119(13):8087-8130
pubmed: 31125213
Nano Lett. 2017 Jun 14;17(6):3710-3717
pubmed: 28481115
ACS Nano. 2021 Feb 23;15(2):2458-2467
pubmed: 32941001
J Phys Chem B. 2021 Nov 11;125(44):12197-12205
pubmed: 34723520
Phys Rev Lett. 2006 May 12;96(18):186101
pubmed: 16712374
Nano Lett. 2018 Feb 14;18(2):874-880
pubmed: 29272135
Nano Lett. 2013 Apr 10;13(4):1736-42
pubmed: 23517407
ACS Nano. 2012 Aug 28;6(8):7177-84
pubmed: 22830934
Nano Lett. 2018 Nov 14;18(11):7289-7297
pubmed: 30352162
J Opt Soc Am A Opt Image Sci Vis. 2019 Nov 1;36(11):C78-C84
pubmed: 31873698
Light Sci Appl. 2020 Jun 28;9:108
pubmed: 32612818
Nat Nanotechnol. 2017 Oct;12(10):1000-1005
pubmed: 28737751
ACS Nano. 2017 Oct 24;11(10):9678-9688
pubmed: 28853862
J Am Chem Soc. 2014 May 14;136(19):6870-3
pubmed: 24779561
ACS Nano. 2012 Mar 27;6(3):2452-8
pubmed: 22305011
Nano Lett. 2010 Nov 10;10(11):4302-8
pubmed: 20925400
ACS Nano. 2020 Apr 28;14(4):5061-5074
pubmed: 32167744
Nano Lett. 2013 Sep 11;13(9):4075-9
pubmed: 23899267
Nano Lett. 2018 Mar 14;18(3):1714-1723
pubmed: 29438619
J Phys Condens Matter. 2017 May 24;29(20):203002
pubmed: 28426435
Nano Lett. 2010 Dec 8;10(12):4794-8
pubmed: 20957994
Sci Adv. 2021 Mar 5;7(10):
pubmed: 33674315
ACS Energy Lett. 2022 Feb 11;7(2):778-815
pubmed: 35178471
ACS Nano. 2013 Sep 24;7(9):7874-85
pubmed: 23971967
Nat Nanotechnol. 2015 Jan;10(1):2-6
pubmed: 25559961
ACS Nano. 2018 Feb 27;12(2):976-985
pubmed: 29283248
ACS Appl Mater Interfaces. 2022 Aug 10;14(31):35734-35744
pubmed: 35913208
Small. 2022 Aug;18(31):e2201602
pubmed: 35789234
Light Sci Appl. 2019 Oct 2;8:89
pubmed: 31645933
ACS Nano. 2017 Dec 26;11(12):12346-12357
pubmed: 29155558
ACS Nano. 2016 Jun 28;10(6):6299-305
pubmed: 27212221
Proc Natl Acad Sci U S A. 2016 Aug 9;113(32):8916-20
pubmed: 27444015
Science. 2018 Oct 5;362(6410):69-72
pubmed: 30287657
Nanoscale. 2019 Nov 7;11(41):19561-19570
pubmed: 31583393
Nano Lett. 2019 Mar 13;19(3):1867-1874
pubmed: 30789274
Nano Lett. 2012 Aug 8;12(8):4385-91
pubmed: 22775068
Nano Lett. 2015 Apr 8;15(4):2600-4
pubmed: 25734469
Nanoscale. 2020 Sep 14;12(34):17870-17879
pubmed: 32840546
Nanoscale. 2015 Jan 14;7(2):577-82
pubmed: 25418974
Nano Lett. 2011 Mar 9;11(3):1061-9
pubmed: 21306114
Nat Mater. 2020 Sep;19(9):946-958
pubmed: 32807918
Annu Rev Phys Chem. 2021 Apr 20;72:99-119
pubmed: 33267646
J Chem Phys. 2022 Jan 21;156(3):034201
pubmed: 35065575
ACS Appl Mater Interfaces. 2020 Dec 2;12(48):53816-53826
pubmed: 33201661
Nat Commun. 2023 Jun 27;14(1):3813
pubmed: 37369657
Nano Lett. 2019 Feb 13;19(2):1067-1073
pubmed: 30657694
ACS Nano. 2018 Aug 28;12(8):8447-8455
pubmed: 30071160
ACS Nano. 2020 Dec 22;14(12):16202-16219
pubmed: 33314905
ACS Nano. 2020 Nov 24;14(11):15757-15765
pubmed: 32852941
Langmuir. 2022 Mar 29;38(12):3876-3886
pubmed: 35302776
Nat Mater. 2015 Jun;14(6):567-76
pubmed: 25990912
Nano Lett. 2016 Feb 10;16(2):1224-9
pubmed: 26745330
Nano Lett. 2013 Jan 9;13(1):240-7
pubmed: 23194158
Annu Rev Phys Chem. 2021 Apr 20;72:423-443
pubmed: 33481640
Acc Chem Res. 2019 Sep 17;52(9):2525-2535
pubmed: 31430119
Angew Chem Int Ed Engl. 2012 Aug 13;51(33):8352-5
pubmed: 22777822