Catalytic Alkyne Semihydrogenation with Polyhydride Ni/Ga Clusters.

(Poly-) Hydrides Density Functional Calculations Metal Cluster ROESY Semihydrogenation Catalysis

Journal

Angewandte Chemie (International ed. in English)
ISSN: 1521-3773
Titre abrégé: Angew Chem Int Ed Engl
Pays: Germany
ID NLM: 0370543

Informations de publication

Date de publication:
04 Sep 2023
Historique:
received: 22 06 2023
medline: 6 7 2023
pubmed: 6 7 2023
entrez: 6 7 2023
Statut: ppublish

Résumé

The bimetallic, decanuclear Ni

Identifiants

pubmed: 37408378
doi: 10.1002/anie.202308790
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e202308790

Subventions

Organisme : Deutsche Forschungsgemeinschaft
ID : FI 502/44-1
Organisme : Grand Équipement National De Calcul Intensif
ID : A0050807367

Informations de copyright

© 2023 The Authors. Angewandte Chemie International Edition published by Wiley-VCH GmbH.

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In a different approach the catalytic activity of TM centres has been modified by positioning a Lewis-acidic E(III) centre in close proximity. This achieved by the use of sophistically tailored pincer-type ligands:
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Deposition number 2180123 contains the supplementary crystallographic data for this paper. These data are provided free of charge by the joint Cambridge Crystallographic Data Centre and Fachinformationszentrum Karlsruhe Access Structures service.

Auteurs

Maximilian Muhr (M)

Technical University of Munich, TUM School of Natural Sciences, Department of Chemistry, Chair of Inorganic and Metal-Organic Chemistry, Lichtenbergstraße 4, 85748, Garching, Germany.
Catalysis Research Centre, Technical University Munich, Ernst-Otto-Fischer Straße 1, 85748, Garching, Germany.

Hao Liang (H)

Univ Rennes, CNRS, ISCR-UMR 6226, 35000, Rennes, France.

Lars Allmendinger (L)

Department of Pharmacy, Ludwig-Maximilians-University Munich, Butenandtstrasse 7, 81377, Munich, Germany.

Raphael Bühler (R)

Technical University of Munich, TUM School of Natural Sciences, Department of Chemistry, Chair of Inorganic and Metal-Organic Chemistry, Lichtenbergstraße 4, 85748, Garching, Germany.
Catalysis Research Centre, Technical University Munich, Ernst-Otto-Fischer Straße 1, 85748, Garching, Germany.

Fabrizio E Napoli (FE)

Technical University of Munich, TUM School of Natural Sciences, Department of Chemistry, Chair of Inorganic and Metal-Organic Chemistry, Lichtenbergstraße 4, 85748, Garching, Germany.
Catalysis Research Centre, Technical University Munich, Ernst-Otto-Fischer Straße 1, 85748, Garching, Germany.

Dardan Ukaj (D)

Technical University of Munich, TUM School of Natural Sciences, Department of Chemistry, Chair of Inorganic and Metal-Organic Chemistry, Lichtenbergstraße 4, 85748, Garching, Germany.
Catalysis Research Centre, Technical University Munich, Ernst-Otto-Fischer Straße 1, 85748, Garching, Germany.

Mirza Cokoja (M)

Technical University of Munich, TUM School of Natural Sciences, Department of Chemistry, Chair of Inorganic and Metal-Organic Chemistry, Lichtenbergstraße 4, 85748, Garching, Germany.
Catalysis Research Centre, Technical University Munich, Ernst-Otto-Fischer Straße 1, 85748, Garching, Germany.

Christian Jandl (C)

Technical University of Munich, TUM School of Natural Sciences, Department of Chemistry, Chair of Inorganic and Metal-Organic Chemistry, Lichtenbergstraße 4, 85748, Garching, Germany.
Catalysis Research Centre, Technical University Munich, Ernst-Otto-Fischer Straße 1, 85748, Garching, Germany.

Samia Kahlal (S)

Univ Rennes, CNRS, ISCR-UMR 6226, 35000, Rennes, France.

Jean-Yves Saillard (JY)

Univ Rennes, CNRS, ISCR-UMR 6226, 35000, Rennes, France.

Christian Gemel (C)

Technical University of Munich, TUM School of Natural Sciences, Department of Chemistry, Chair of Inorganic and Metal-Organic Chemistry, Lichtenbergstraße 4, 85748, Garching, Germany.
Catalysis Research Centre, Technical University Munich, Ernst-Otto-Fischer Straße 1, 85748, Garching, Germany.

Roland A Fischer (RA)

Technical University of Munich, TUM School of Natural Sciences, Department of Chemistry, Chair of Inorganic and Metal-Organic Chemistry, Lichtenbergstraße 4, 85748, Garching, Germany.
Catalysis Research Centre, Technical University Munich, Ernst-Otto-Fischer Straße 1, 85748, Garching, Germany.

Classifications MeSH