Antimalarial Agents Derived from Metal-Amodiaquine Complexes with Activity in Multiple Stages of the Plasmodium Life Cycle.


Journal

Chemistry (Weinheim an der Bergstrasse, Germany)
ISSN: 1521-3765
Titre abrégé: Chemistry
Pays: Germany
ID NLM: 9513783

Informations de publication

Date de publication:
02 Oct 2023
Historique:
received: 23 05 2023
medline: 4 10 2023
pubmed: 10 7 2023
entrez: 10 7 2023
Statut: ppublish

Résumé

Malaria is the one of the deadliest infectious diseases worldwide. Chemically, quinolines are excellent ligands for metal coordination and are deployed as drugs for malaria treatment. There is a growing body of evidence indicating that metal complexes can be conjugated with antimalarial quinolines to be used as chemical tools to overcome the disadvantages of quinolines, improving their bioactive speciation, cellular distribution, and subsequently broadening the spectrum of activity to multiple stages of the complex Plasmodium life cycle. In this study, four novel complexes of ruthenium(II)- and gold(I)-containing amodiaquine (AQ) were synthesized, and a careful chemical characterization revealed the precise coordination site of AQ to the metals. Their speciation in solution was investigated, demonstrating the stability of the quinoline-metal bond. Ru

Identifiants

pubmed: 37427863
doi: 10.1002/chem.202301642
doi:

Substances chimiques

Antimalarials 0
Amodiaquine 220236ED28
Coordination Complexes 0
Quinolines 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e202301642

Subventions

Organisme : Fundação de Amparo à Pesquisa do Estado do Rio Grande do Sul
ID : 54829.632.62060.05032021
Organisme : Fundação de Amparo à Pesquisa do Estado de São Paulo
ID : 16/23130-5, 21/02522-0, and 17/15850-0
Organisme : Conselho Nacional de Desenvolvimento Científico e Tecnológico
ID : 305388/2022-3
Organisme : Fundação Oswaldo Cruz
ID : 002-FIO-20-2-25

Informations de copyright

© 2023 Wiley-VCH GmbH.

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Auteurs

Legna Colina-Vegas (L)

Instituto de Química, Universidade Federal do Rio Grande do Sul, Porto Alegre, CP 91501-970, RS, Brazil.

Mariana da Cruz B Silva (M)

Instituto Gonçalo Moniz, FIOCRUZ, Salvador, CEP 40296-710, BA, Brazil.

Caroline de Souza Pereira (C)

Departamento de Química, Universidade Federal de Juiz de Fora, Juiz de Fora, CP 36036-900, MG, Brazil.

Ariane Isis Barros (A)

Departamento de Solos e Engenharia Rural, Universidade Federal de Mato Grosso, Cuiabá, CEP 78060-900, MT, Brazil.

Joaquim Araújo Nobrega (J)

Departamento de Química, Universidade Federal de São Carlos, São Carlos, CP 13565-90, SP, Brazil.

Maribel Navarro (M)

Departamento de Química, Universidade Federal de Juiz de Fora, Juiz de Fora, CP 36036-900, MG, Brazil.

Matthias Rottmann (M)

Swiss Tropical & Public Health Institute, 4123, Allschwil, Switzerland.
University of Basel, 4001, Basel, Switzerland.

Sarah D'Alessandro (S)

Dipartimento di Scienze Farmacologiche e Biomolecolari, Università degli Studi di Milano, Milan, 20133, Italy.

Nicoletta Basilico (N)

Dipartimento di Scienze Biomediche, Chirurgiche e Odontoiatriche, Universitá degli Studi di Milano, Milan, 20133, Italy.

Alzir Azevedo Batista (A)

Departamento de Química, Universidade Federal de São Carlos, São Carlos, CP 13565-90, SP, Brazil.

Diogo R M Moreira (DRM)

Instituto Gonçalo Moniz, FIOCRUZ, Salvador, CEP 40296-710, BA, Brazil.

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