Geochemical Integrity of Wellbore Cements during Geological Hydrogen Storage.


Journal

Environmental science & technology letters
ISSN: 2328-8930
Titre abrégé: Environ Sci Technol Lett
Pays: United States
ID NLM: 101628367

Informations de publication

Date de publication:
11 Jul 2023
Historique:
received: 11 05 2023
revised: 12 06 2023
accepted: 12 06 2023
medline: 17 7 2023
pubmed: 17 7 2023
entrez: 17 7 2023
Statut: epublish

Résumé

Increasing greenhouse gas emissions have put pressure on global economies to adopt strategies for climate-change mitigation. Large-scale geological hydrogen storage in salt caverns and porous rocks has the potential to achieve sustainable energy storage, contributing to the development of a low-carbon economy. During geological storage, hydrogen is injected and extracted through cemented and cased wells. In this context, well integrity and leakage risk must be assessed through in-depth investigations of the hydrogen-cement-rock physical and geochemical processes. There are significant scientific knowledge gaps pertaining to hydrogen-cement interactions, where chemical reactions among hydrogen, in situ reservoir fluids, and cement could degrade the well cement and put the integrity of the storage system at risk. Results from laboratory batch reaction experiments concerning the influence of hydrogen on cement samples under simulated reservoir conditions of North Sea fields, including temperature, pressure, and salinity, provided valuable insights into the integrity of cement for geological hydrogen storage. This work shows that, under the experimental conditions, hydrogen does not induce geochemical or structural alterations to the tested wellbore cements, a promising finding for secure hydrogen subsurface storage.

Identifiants

pubmed: 37455863
doi: 10.1021/acs.estlett.3c00303
pmc: PMC10339721
doi:

Types de publication

Journal Article

Langues

eng

Pagination

551-556

Informations de copyright

© 2023 The Authors. Published by American Chemical Society.

Déclaration de conflit d'intérêts

The authors declare no competing financial interest.

Références

Environ Sci Technol. 2015 May 19;49(10):6335-43
pubmed: 25893278
ACS Energy Lett. 2022 Jul 8;7(7):2203-2210
pubmed: 35844470

Auteurs

Adnan Aftab (A)

School of Geosciences, University of Edinburgh, Grant Institute, West Main Road, Edinburgh EH9 3FE, United Kingdom.
Curtin University, Discipline of Petroleum Engineering, 26 Dick Perry Avenue, 6151 Kensington, Australia.

Aliakbar Hassanpouryouzband (A)

School of Geosciences, University of Edinburgh, Grant Institute, West Main Road, Edinburgh EH9 3FE, United Kingdom.

Abby Martin (A)

School of Geosciences, University of Edinburgh, Grant Institute, West Main Road, Edinburgh EH9 3FE, United Kingdom.

Jackie E Kendrick (JE)

School of Geosciences, University of Edinburgh, Grant Institute, West Main Road, Edinburgh EH9 3FE, United Kingdom.
Department of Earth and Environmental Science, Ludwig Maximilian University, Theresienstrasse 41, 80333 Munich, Germany.

Eike M Thaysen (EM)

School of Geosciences, University of Edinburgh, Grant Institute, West Main Road, Edinburgh EH9 3FE, United Kingdom.
Department of Geosciences, Institute of Environmental Assessment and Water Research (IDAEA), Severo Ochoa Excellence Center of the Spanish Council for Scientific Research (CSIC), Jordi Girona 18-26, 08034 Barcelona, Spain.

Niklas Heinemann (N)

School of Geosciences, University of Edinburgh, Grant Institute, West Main Road, Edinburgh EH9 3FE, United Kingdom.

James Utley (J)

School of Environmental Sciences, University of Liverpool, 4 Brownlow Street, Liverpool L69 3GP, United Kingdom.

Mark Wilkinson (M)

School of Geosciences, University of Edinburgh, Grant Institute, West Main Road, Edinburgh EH9 3FE, United Kingdom.

R Stuart Haszeldine (RS)

School of Geosciences, University of Edinburgh, Grant Institute, West Main Road, Edinburgh EH9 3FE, United Kingdom.

Katriona Edlmann (K)

School of Geosciences, University of Edinburgh, Grant Institute, West Main Road, Edinburgh EH9 3FE, United Kingdom.

Classifications MeSH