Efficient noble metal promoted bimetallic cobalt catalysts in the selective synthesis of acetaldehyde dimethyl acetal.


Journal

RSC advances
ISSN: 2046-2069
Titre abrégé: RSC Adv
Pays: England
ID NLM: 101581657

Informations de publication

Date de publication:
26 Jul 2023
Historique:
received: 27 04 2023
accepted: 29 06 2023
medline: 28 7 2023
pubmed: 28 7 2023
entrez: 28 7 2023
Statut: epublish

Résumé

Herein we report the one-pot cobalt catalysed synthesis of the dimethylacetal of acetaldehyde from synthesis gas and methanol. The product can be used as a fuel additive either as it is or after transacetalisation with long-chain alcohols. The product is obtained at moderate temperatures in good selectivities and high CO-conversions. A variation of the promotor metal (Au, Pt, Pd, and Ru) and of the support (γ-Al

Identifiants

pubmed: 37502823
doi: 10.1039/d3ra02784h
pii: d3ra02784h
pmc: PMC10369129
doi:

Types de publication

Journal Article

Langues

eng

Pagination

22698-22709

Informations de copyright

This journal is © The Royal Society of Chemistry.

Déclaration de conflit d'intérêts

There are no conflicts to declare.

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Auteurs

Kalim A Sheikh (KA)

Karlsruher Institut für Technologie (KIT) Eggenstein-Leopoldshafen Germany kalim.sheikh@kit.edu thomas.zevaco@kit.edu.
BASF SE Ludwigshafen Germany.

Thomas A Zevaco (TA)

Karlsruher Institut für Technologie (KIT) Eggenstein-Leopoldshafen Germany kalim.sheikh@kit.edu thomas.zevaco@kit.edu.

Jelena Jelic (J)

Karlsruher Institut für Technologie (KIT) Eggenstein-Leopoldshafen Germany kalim.sheikh@kit.edu thomas.zevaco@kit.edu.

Felix Studt (F)

Karlsruher Institut für Technologie (KIT) Eggenstein-Leopoldshafen Germany kalim.sheikh@kit.edu thomas.zevaco@kit.edu.

Michael Bender (M)

BASF SE Ludwigshafen Germany.

Classifications MeSH