Experimental Evidence for Double Quaternary Azeotropy's Existence.

azeotropy rule double azeotropy phase diagram quaternary system singular points vapor‒liquid equilibrium

Journal

Entropy (Basel, Switzerland)
ISSN: 1099-4300
Titre abrégé: Entropy (Basel)
Pays: Switzerland
ID NLM: 101243874

Informations de publication

Date de publication:
26 Jun 2023
Historique:
received: 30 05 2023
revised: 09 06 2023
accepted: 25 06 2023
medline: 29 7 2023
pubmed: 29 7 2023
entrez: 29 7 2023
Statut: epublish

Résumé

The phase equilibrium in an acetonitrile + water + cyclohexene + chloroform system was studied at 101.3 kPa. A prediction regarding the internal structure of the composition tetrahedron (presence/absence of one/two internal singular points) was made using thermodynamic modeling in AspenPlus V.10.0. The existence of two internal quaternary azeotropes (of node type with a minimum boiling point and of saddle type) was confirmed as a result of a full-scale experiment. Thermodynamic-topological analysis of the structure of phase equilibrium diagrams was carried out to confirm the correctness of the diagram construction.

Identifiants

pubmed: 37509927
pii: e25070980
doi: 10.3390/e25070980
pmc: PMC10377813
pii:
doi:

Types de publication

Journal Article

Langues

eng

Subventions

Organisme : Ministry of Education and Science in the framework of the State task
ID : FSFZ-2023-0003

Références

Talanta. 1985 Aug;32(8 Pt 2):735-43
pubmed: 18963997

Auteurs

Anastasia Frolkova (A)

Lomonosov Institute of Fine Chemical Technologies, MIREA-Russian Technological University, 119454 Moscow, Russia.

Valeriy Zhuchkov (V)

Lomonosov Institute of Fine Chemical Technologies, MIREA-Russian Technological University, 119454 Moscow, Russia.

Alla Frolkova (A)

Lomonosov Institute of Fine Chemical Technologies, MIREA-Russian Technological University, 119454 Moscow, Russia.

Classifications MeSH