Antibubbles Enable Tunable Payload Release with Low-Intensity Ultrasound.

antibubbles low-intensity ultrasound payload smart materials triggered release

Journal

Advanced materials (Deerfield Beach, Fla.)
ISSN: 1521-4095
Titre abrégé: Adv Mater
Pays: Germany
ID NLM: 9885358

Informations de publication

Date de publication:
Nov 2023
Historique:
revised: 25 07 2023
received: 03 06 2023
medline: 29 11 2023
pubmed: 29 7 2023
entrez: 29 7 2023
Statut: ppublish

Résumé

The benefits of ultrasound are its ease-of-use and its ability to precisely deliver energy in opaque and complex media. However, most materials responsive to ultrasound show a weak response, requiring the use of high powers, which are associated with undesirable streaming, cavitation, or temperature rise. These effects hinder response control and may even cause damage to the medium where the ultrasound is applied. Moreover, materials that are currently in use rely on all-or-nothing effects, limiting the ability to fine-tune the response of the material on the fly. For these reasons, there is a need for materials that can respond to low intensity ultrasound with programmable responses. Here it is demonstrated that antibubbles are a low-intensity-ultrasound-responsive material system that can controllably release a payload using acoustic pressures in the kilopascal range. Varying their size and composition tunes the release pressure, and the response can be switched between a single release and stepwise release across multiple ultrasound pulses. Observations using confocal and high-speed microscopy reveal different ways that can lead to release. These findings lay the groundwork to design antibubbles that controllably respond to low-intensity ultrasound, opening a wide range of applications ranging from ultrasound-responsive material systems to carriers for targeted delivery.

Identifiants

pubmed: 37515825
doi: 10.1002/adma.202305296
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

e2305296

Subventions

Organisme : European Research Council
ID : 788296
Pays : International

Informations de copyright

© 2023 The Authors. Advanced Materials published by Wiley-VCH GmbH.

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Auteurs

Nicolas Moreno-Gomez (N)

Institute for Molecular Systems Engineering and Advanced Materials, Heidelberg University, Im Neuenheimer Feld 225, 69120, Heidelberg, Germany.
Max Planck Institute for Medical Research, Jahnstr. 29, 69120, Heidelberg, Germany.

Athanasios G Athanassiadis (AG)

Institute for Molecular Systems Engineering and Advanced Materials, Heidelberg University, Im Neuenheimer Feld 225, 69120, Heidelberg, Germany.
Max Planck Institute for Medical Research, Jahnstr. 29, 69120, Heidelberg, Germany.

Albert T Poortinga (AT)

Polymer Technology Group, Eindhoven University of Technology, De Rondom 70, Eindhoven, 5612 AZ, The Netherlands.

Peer Fischer (P)

Institute for Molecular Systems Engineering and Advanced Materials, Heidelberg University, Im Neuenheimer Feld 225, 69120, Heidelberg, Germany.
Max Planck Institute for Medical Research, Jahnstr. 29, 69120, Heidelberg, Germany.

Classifications MeSH