Data Science Enables the Development of a New Class of Chiral Phosphoric Acid Catalysts.


Journal

Chem
ISSN: 2451-9294
Titre abrégé: Chem
Pays: United States
ID NLM: 101688902

Informations de publication

Date de publication:
08 Jun 2023
Historique:
pmc-release: 08 06 2024
medline: 31 7 2023
pubmed: 31 7 2023
entrez: 31 7 2023
Statut: ppublish

Résumé

The widespread success of BINOL-chiral phosphoric acids (CPAs) has led to the development of several high molecular weight, sterically encumbered variants. Herein, we disclose an alternative, minimalistic chiral phosphoric acid backbone incorporating only a single instance of point chirality. Data science techniques were used to select a diverse training set of catalysts, which were benchmarked against the transfer hydrogenation of an 8-aminoquinoline. Using a univariate classification algorithm and multivariate linear regression, key catalyst features necessary for high levels of selectivity were deconvoluted, revealing a simple catalyst model capable of predicting selectivity for out-of-set catalysts. This workflow enabled extrapolation to a catalyst providing higher selectivity than both reported peptide-type and BINOL-type catalysts (up to 95:5

Identifiants

pubmed: 37519827
doi: 10.1016/j.chempr.2023.02.020
pmc: PMC10373836
mid: NIHMS1881262
doi:

Types de publication

Journal Article

Langues

eng

Pagination

1518-1537

Subventions

Organisme : NIGMS NIH HHS
ID : R35 GM136271
Pays : United States

Déclaration de conflit d'intérêts

DECLARATION OF INTERESTS The authors declare no competing interests.

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Auteurs

Jordan P Liles (JP)

Department of Chemistry, University of Utah, 315 S 1400 E, Salt Lake City, UT, 84112, USA.

Caroline Rouget-Virbel (C)

College of Chemistry, University of California, Berkeley, Berkeley, CA, 94720, USA.

Julie L H Wahlman (JLH)

Department of Chemistry, University of Utah, 315 S 1400 E, Salt Lake City, UT, 84112, USA.

Rene Rahimoff (R)

College of Chemistry, University of California, Berkeley, Berkeley, CA, 94720, USA.

Jennifer M Crawford (JM)

Department of Chemistry, University of Utah, 315 S 1400 E, Salt Lake City, UT, 84112, USA.

Abby Medlin (A)

College of Chemistry, University of California, Berkeley, Berkeley, CA, 94720, USA.

Veronica O'Connor (V)

Department of Chemistry, University of Utah, 315 S 1400 E, Salt Lake City, UT, 84112, USA.

Junqi Li (J)

College of Chemistry, University of California, Berkeley, Berkeley, CA, 94720, USA.

Vladislav A Roytman (VA)

College of Chemistry, University of California, Berkeley, Berkeley, CA, 94720, USA.

F Dean Toste (FD)

College of Chemistry, University of California, Berkeley, Berkeley, CA, 94720, USA.

Matthew S Sigman (MS)

Department of Chemistry, University of Utah, 315 S 1400 E, Salt Lake City, UT, 84112, USA.
Lead contact.

Classifications MeSH