Facile and Cost-effective Synthesis of CoP@N-doped Carbon with High Catalytic Performance for Electrochemical Hydrogen Evolution Reaction.
Carbon materials
Electrocatalysts
Hydrogen evolution reaction
Transition metal catalyst
Journal
Chemistry, an Asian journal
ISSN: 1861-471X
Titre abrégé: Chem Asian J
Pays: Germany
ID NLM: 101294643
Informations de publication
Date de publication:
17 Oct 2023
17 Oct 2023
Historique:
revised:
25
07
2023
received:
19
06
2023
medline:
7
8
2023
pubmed:
7
8
2023
entrez:
7
8
2023
Statut:
ppublish
Résumé
The manufacture of efficient and low-cost hydrogen evolution reaction (HER) catalysts is regarded as a critical solution to achieve carbon neutrality. Herein, we developed an economical method to synthesize a CoP-anchored N-doped carbon catalyst via one-step pyrolysis using inexpensive starting materials (cobalt ion salt, phytic acid, and glycine). The size of the CoP nanoparticles was controlled by adjusting the Co/P ratio of the catalysts. Nanoscale CoP particles with adequate exposure to active sites were uniformly anchored on the surface of the conductive nitrogen-doped carbon substrate, ensuring the rapid transfer of electrons and species. When Co/P=0.89, the as-made catalyst exhibited outstanding HER activity, with an extraordinarily low overpotential of 202 mV at 10 mA cm
Identifiants
pubmed: 37545336
doi: 10.1002/asia.202300534
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e202300534Subventions
Organisme : Research Center for Ultra-High Voltage Electron Microscopy, Osaka University
Informations de copyright
© 2023 Wiley-VCH GmbH.
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